Tunable Orthogonal Reversible Covalent (TORC) Bonds: Dynamic Chemical Control over Molecular Assembly.

dynamic covalent chemistry dynamic materials molecular assembly molecular recognition orthogonality

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
02 01 2019
Historique:
received: 21 07 2018
pubmed: 12 8 2018
medline: 1 8 2020
entrez: 12 8 2018
Statut: ppublish

Résumé

Dynamic assembly of macromolecules in biological systems is one of the fundamental processes that facilitates life. Although such assembly most commonly uses noncovalent interactions, a set of dynamic reactions involving reversible covalent bonding is actively being exploited for the design of functional materials, bottom-up assembly, and molecular machines. This Minireview highlights recent implementations and advancements in the area of tunable orthogonal reversible covalent (TORC) bonds for these purposes, and provides an outlook for their expansion, including the development of synthetically encoded polynucleotide mimics.

Identifiants

pubmed: 30098086
doi: 10.1002/anie.201808371
doi:

Substances chimiques

Macromolecular Substances 0

Types de publication

Journal Article Research Support, N.I.H., Extramural Research Support, Non-U.S. Gov't Research Support, U.S. Gov't, Non-P.H.S. Review

Langues

eng

Sous-ensembles de citation

IM

Pagination

74-85

Subventions

Organisme : Division of Materials Research
ID : DMR-1720595
Pays : International
Organisme : Defense Advanced Research Projects Agency
ID : N66001-14-2-4051
Pays : International
Organisme : Welch Foundation
ID : F-0046
Pays : International
Organisme : NIH HHS
ID : 1R01EB022025-01A1
Pays : United States

Informations de copyright

© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Auteurs

James F Reuther (JF)

Department of Chemistry, University of Texas at Austin, Austin, TX, USA.
Department of Chemistry, University of Massachusetts Lowell, Lowell, MA, USA.

Samuel D Dahlhauser (SD)

Department of Chemistry, University of Texas at Austin, Austin, TX, USA.

Eric V Anslyn (EV)

Department of Chemistry, University of Texas at Austin, Austin, TX, USA.

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Classifications MeSH