C-I-Selective Cross-Coupling Enabled by a Cationic Palladium Trimer.

C−C bond formation chemoselectivity cross-coupling density functional calculations palladium trimers

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
02 Jan 2019
Historique:
received: 04 10 2018
pubmed: 2 11 2018
medline: 2 11 2018
entrez: 2 11 2018
Statut: ppublish

Résumé

While there is a growing interest in harnessing synergistic effects of more than one metal in catalysis, relatively little is known beyond bimetallic systems. This report describes the straightforward access to an air-stable Pd trimer and presents unambiguous reactivity data of its privileged capability to differentiate C-I over C-Br bonds in C-C bond formations (arylation and alkylation) of polyhalogenated arenes, which typical Pd

Identifiants

pubmed: 30381881
doi: 10.1002/anie.201811380
doi:

Types de publication

Journal Article

Langues

eng

Pagination

211-215

Subventions

Organisme : H2020 European Research Council
ID : ERC-637993

Informations de copyright

© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Auteurs

Claudia J Diehl (CJ)

Institute of Organic Chemistry, RWTH Aachen University, Landoltweg 1, 52074, Aachen, Germany.

Thomas Scattolin (T)

Institute of Organic Chemistry, RWTH Aachen University, Landoltweg 1, 52074, Aachen, Germany.

Ulli Englert (U)

Institute of Organic Chemistry, RWTH Aachen University, Landoltweg 1, 52074, Aachen, Germany.

Franziska Schoenebeck (F)

Institute of Organic Chemistry, RWTH Aachen University, Landoltweg 1, 52074, Aachen, Germany.

Classifications MeSH