First-principles modeling of water permeation through periodically porous graphene derivatives.

Covalent triazine framework (CTF) Density functional theory (DFT) Hydrogen bonding Nanoporous membrane Polyphenylene superhoneycomb network (PSN) Porous graphene Water permeation

Journal

Journal of colloid and interface science
ISSN: 1095-7103
Titre abrégé: J Colloid Interface Sci
Pays: United States
ID NLM: 0043125

Informations de publication

Date de publication:
07 Mar 2019
Historique:
received: 22 10 2018
revised: 27 11 2018
accepted: 28 11 2018
pubmed: 12 12 2018
medline: 12 12 2018
entrez: 12 12 2018
Statut: ppublish

Résumé

Polyphenylene superhoneycomb network (PSN) and covalent triazine framework (CTF) are experimentally realized periodically porous graphene derivatives. Such ultrathin layers with homogeneously distributed pores of controllable sizes are highly desirable for applications in molecular separations such as water purification. The permeation energy barrier is expected to be a function of not only the pore size, but also the specific permeation trajectory as determined by hydrogen bonding interactions at the water-pore interface. Here, we report a detailed first-principles study of permeation of a single H

Identifiants

pubmed: 30530034
pii: S0021-9797(18)31428-0
doi: 10.1016/j.jcis.2018.11.106
pii:
doi:

Types de publication

Journal Article

Langues

eng

Pagination

367-376

Informations de copyright

Copyright © 2018 Elsevier Inc. All rights reserved.

Auteurs

Jin Soo Lim (JS)

Department of Chemistry and Chemical Biology, Harvard University, Cambridge MA 02138, USA. Electronic address: limjs@g.harvard.edu.

Gunn Kim (G)

Department of Physics and Astronomy, Sejong University, Seoul 143-747, South Korea; Graphene Research Institute, Sejong University, Seoul 143-747, South Korea. Electronic address: gunnkim@sejong.ac.kr.

Classifications MeSH