Complete steric exclusion of ions and proton transport through confined monolayer water.


Journal

Science (New York, N.Y.)
ISSN: 1095-9203
Titre abrégé: Science
Pays: United States
ID NLM: 0404511

Informations de publication

Date de publication:
11 01 2019
Historique:
received: 05 07 2018
accepted: 23 11 2018
entrez: 12 1 2019
pubmed: 12 1 2019
medline: 12 1 2019
Statut: ppublish

Résumé

It has long been an aspirational goal to create artificial structures that allow fast permeation of water but reject even the smallest hydrated ions, replicating the feat achieved by nature in protein channels (e.g., aquaporins). Despite recent progress in creating nanoscale pores and capillaries, these structures still remain distinctly larger than protein channels. We report capillaries made by effectively extracting one atomic plane from bulk crystals, which leaves a two-dimensional slit of a few angstroms in height. Water moves through these capillaries with little resistance, whereas no permeation could be detected even for such small ions as Na

Identifiants

pubmed: 30630924
pii: 363/6423/145
doi: 10.1126/science.aau6771
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Pagination

145-148

Subventions

Organisme : European Research Council
Pays : International

Informations de copyright

Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.

Auteurs

K Gopinadhan (K)

School of Physics and Astronomy, University of Manchester, Manchester M13 9PL, UK.
National Graphene Institute, University of Manchester, Manchester M13 9PL, UK.
Department of Physics, Indian Institute of Technology Gandhinagar, Gujarat 382355, India.

S Hu (S)

National Graphene Institute, University of Manchester, Manchester M13 9PL, UK.

A Esfandiar (A)

School of Physics and Astronomy, University of Manchester, Manchester M13 9PL, UK.
Department of Physics, Sharif University of Technology, P.O. Box 11155-9161, Tehran, Iran.

M Lozada-Hidalgo (M)

School of Physics and Astronomy, University of Manchester, Manchester M13 9PL, UK.

F C Wang (FC)

School of Physics and Astronomy, University of Manchester, Manchester M13 9PL, UK.
Chinese Academy of Sciences Key Laboratory of Mechanical Behavior and Design of Materials, Department of Modern Mechanics, University of Science and Technology of China, Hefei, Anhui 230027, China.

Q Yang (Q)

National Graphene Institute, University of Manchester, Manchester M13 9PL, UK.
Key Laboratory of Advanced Technologies of Materials, School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu, Sichuan 610031, China.

A V Tyurnina (AV)

National Graphene Institute, University of Manchester, Manchester M13 9PL, UK.
Skolkovo Institute of Science and Technology, Nobel St. 3, 143026 Moscow, Russia.

A Keerthi (A)

School of Physics and Astronomy, University of Manchester, Manchester M13 9PL, UK.
National Graphene Institute, University of Manchester, Manchester M13 9PL, UK.

B Radha (B)

School of Physics and Astronomy, University of Manchester, Manchester M13 9PL, UK. geim@manchester.ac.uk radha.boya@manchester.ac.uk.
National Graphene Institute, University of Manchester, Manchester M13 9PL, UK.

A K Geim (AK)

School of Physics and Astronomy, University of Manchester, Manchester M13 9PL, UK. geim@manchester.ac.uk radha.boya@manchester.ac.uk.
National Graphene Institute, University of Manchester, Manchester M13 9PL, UK.

Classifications MeSH