New thiazol-hydrazono-coumarin hybrids targeting human cervical cancer cells: Synthesis, CDK2 inhibition, QSAR and molecular docking studies.


Journal

Bioorganic chemistry
ISSN: 1090-2120
Titre abrégé: Bioorg Chem
Pays: United States
ID NLM: 1303703

Informations de publication

Date de publication:
05 2019
Historique:
received: 13 07 2018
revised: 18 12 2018
accepted: 16 01 2019
pubmed: 28 1 2019
medline: 1 4 2020
entrez: 28 1 2019
Statut: ppublish

Résumé

Motivated by the potential anticancer activity of both coumarin and 2-aminothiazole nuclei, a new set of thiazol-2-yl hydrazono-chromen-2-one analogs were efficiently synthesized aiming to obtain novel hybrids with potential cytotoxic activity. MTT assay investigated the significant potency of all the target compounds against the human cervical cancer cell lines (HeLa cells). Cell cycle analysis showed that the representative compound 8a led to cell cycle cessation at G0/G1 phase indicating that CDK2/E1complex could be the plausible biological target for these newly synthesized compounds. Thus, the most active compounds (7c and 8a-c) were tested for their CDK2 inhibitory activity. The biological results revealed their significant CDK2 inhibitory activity with IC

Identifiants

pubmed: 30685646
pii: S0045-2068(18)30713-2
doi: 10.1016/j.bioorg.2019.01.026
pii:
doi:

Substances chimiques

Antineoplastic Agents 0
Coumarins 0
Hydrazones 0
Protein Kinase Inhibitors 0
Thiazoles 0
coumarin A4VZ22K1WT
CDK2 protein, human EC 2.7.11.22
Cyclin-Dependent Kinase 2 EC 2.7.11.22

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

80-96

Informations de copyright

Copyright © 2019 Elsevier Inc. All rights reserved.

Auteurs

Somaia S Abd El-Karim (SS)

Therapeutical Chemistry Department, National Research Centre, Dokki, Cairo, P. O. Box 12622, Egypt.

Yasmin M Syam (YM)

Therapeutical Chemistry Department, National Research Centre, Dokki, Cairo, P. O. Box 12622, Egypt. Electronic address: yasmin_syam@yahoo.com.

Ahmed M El Kerdawy (AM)

Department of Pharmaceutical Chemistry, Faculty of Pharmacy, Cairo University, Kasr El-Aini Street, Cairo, P.O. Box 11562, Egypt; Molecular Modeling Unit, Faculty of Pharmacy, Cairo University, Kasr El-Aini Street, Cairo, P.O. Box 11562, Egypt; Department of Pharmaceutical Chemistry, Faculty of Pharmacy, New Giza University, Newgiza, km 22 Cairo-Alexandria Desert Road, Cairo, Egypt.

Tamer M Abdelghany (TM)

Department of Pharmacology, Faculty of Pharmacy, Al-Azhar University, Nasr City, Cairo, P.O. Box 11787, Egypt.

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Classifications MeSH