Merging transformation optics with electron-driven photon sources.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
05 02 2019
Historique:
received: 25 08 2018
accepted: 10 01 2019
entrez: 7 2 2019
pubmed: 7 2 2019
medline: 7 2 2019
Statut: epublish

Résumé

Relativistic electron beams create optical radiation when interacting with tailored nanostructures. This phenomenon has been so far used to design grating-based and holographic electron-driven photon sources. It has been proposed recently that such sources can be used for hybrid electron- and light-based spectroscopy techniques. However, this demands the design of a thin-film source suitable for electron-microscopy applications. Here, we present a mesoscopic structure composed of an array of nanoscale holes in a gold film which is designed using transformation optics and delivers ultrashort chirped electromagnetic wave packets upon 30-200 keV electron irradiation. The femtosecond photon bunches result from coherent scattering of surface plasmon polaritons with hyperbolic dispersion. They decay by radiation in a broad spectral band which is focused into a 1.5 micrometer beam waist. The focusing ability and broadband nature of this photon source will initiate applications in ultrafast spectral interferometry techniques.

Identifiants

pubmed: 30723196
doi: 10.1038/s41467-019-08488-4
pii: 10.1038/s41467-019-08488-4
pmc: PMC6363763
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Pagination

599

Références

J Chem Phys. 2006 Oct 28;125(16):164705
pubmed: 17092118
Opt Express. 2012 Jan 16;20(2):1392-405
pubmed: 22274484
Nature. 2001 Nov 8;414(6860):184-8
pubmed: 11700552
Sci Rep. 2013;3:1903
pubmed: 23712699
Sci Rep. 2016 Sep 21;6:33874
pubmed: 27649932
Nat Commun. 2015 May 05;6:7059
pubmed: 25940659
Nano Lett. 2011 Sep 14;11(9):3779-84
pubmed: 21780758
Science. 2012 Aug 3;337(6094):549-52
pubmed: 22859483
Science. 2011 Jun 10;332(6035):1291-4
pubmed: 21659598
Phys Rev Lett. 2008 Mar 14;100(10):106804
pubmed: 18352220
Phys Rev Lett. 2012 Nov 21;109(21):217401
pubmed: 23215613
Analyst. 2010 Jun;135(6):1175-81
pubmed: 20498870
Sci Rep. 2016 Sep 12;6:32867
pubmed: 27615519
Nat Mater. 2010 Feb;9(2):129-32
pubmed: 20023631
Nature. 2006 Mar 23;440(7083):508-11
pubmed: 16554814
Ultramicroscopy. 2017 May;176:63-73
pubmed: 28139341
Microsc Microanal. 2006 Dec;12(6):506-14
pubmed: 19830943
Nat Commun. 2016 Dec 02;7:13705
pubmed: 27910853
Science. 1966 Oct 21;154(3747):386-8
pubmed: 17751706
Nat Commun. 2018 Jul 12;9(1):2694
pubmed: 30002367

Auteurs

Nahid Talebi (N)

Stuttgart Center for Electron Microscopy, Max Planck Institute for Solid State Research, Heisenbergstr. 1, Stuttgart, 70569, Germany. n.talebi@fkf.mpg.de.

Sophie Meuret (S)

Center for Nanophotonics, AMOLF, Science Park 104, Amsterdam, 1098 XG, The Netherlands.

Surong Guo (S)

Stuttgart Center for Electron Microscopy, Max Planck Institute for Solid State Research, Heisenbergstr. 1, Stuttgart, 70569, Germany.

Mario Hentschel (M)

4th Physics Institute and Research Center SCoPE, University of Stuttgart, Pfaffenwaldring 57, Stuttgart, 70569, Germany.

Albert Polman (A)

Center for Nanophotonics, AMOLF, Science Park 104, Amsterdam, 1098 XG, The Netherlands.

Harald Giessen (H)

4th Physics Institute and Research Center SCoPE, University of Stuttgart, Pfaffenwaldring 57, Stuttgart, 70569, Germany.

Peter A van Aken (PA)

Stuttgart Center for Electron Microscopy, Max Planck Institute for Solid State Research, Heisenbergstr. 1, Stuttgart, 70569, Germany.

Classifications MeSH