Supported Cobalt Nanoparticles for Hydroformylation Reactions.

aldehydes carbonylation cobalt heterogeneous catalysis hydroformylation leaching

Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
11 Apr 2019
Historique:
received: 19 12 2018
pubmed: 20 2 2019
medline: 20 2 2019
entrez: 20 2 2019
Statut: ppublish

Résumé

Hydroformylation of olefins has been studied in the presence of specific heterogeneous cobalt nanoparticles. The catalytic materials were prepared by pyrolysis of preformed cobalt complexes deposited onto different inorganic supports. Atomic absorption spectroscopy (AAS) measurements indicated a correlation of catalyst activity and cobalt leaching as well as a strong influence of the heterogeneous support on the productivity. These new, low-cost, easy-to-handle catalysts can substitute more toxic, unstable and volatile cobalt carbonyl complexes for hydroformylations on a laboratory scale.

Identifiants

pubmed: 30779224
doi: 10.1002/chem.201806282
doi:

Types de publication

Journal Article

Langues

eng

Pagination

5534-5538

Subventions

Organisme : H2020 European Research Council
ID : NoNaCat
Organisme : Bundesministerium für Bildung und Forschung
ID : KataPlasma

Informations de copyright

© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Auteurs

Maximilian Franz Hertrich (MF)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein-Straße 29a, 18059, Rostock, Germany.

Florian Korbinian Scharnagl (FK)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein-Straße 29a, 18059, Rostock, Germany.

Anahit Pews-Davtyan (A)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein-Straße 29a, 18059, Rostock, Germany.

Carsten Robert Kreyenschulte (CR)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein-Straße 29a, 18059, Rostock, Germany.

Henrik Lund (H)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein-Straße 29a, 18059, Rostock, Germany.

Stephan Bartling (S)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein-Straße 29a, 18059, Rostock, Germany.

Ralf Jackstell (R)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein-Straße 29a, 18059, Rostock, Germany.

Matthias Beller (M)

Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein-Straße 29a, 18059, Rostock, Germany.

Classifications MeSH