A nanofluidic ion regulation membrane with aligned cellulose nanofibers.


Journal

Science advances
ISSN: 2375-2548
Titre abrégé: Sci Adv
Pays: United States
ID NLM: 101653440

Informations de publication

Date de publication:
Feb 2019
Historique:
received: 11 06 2018
accepted: 11 01 2019
entrez: 26 2 2019
pubmed: 26 2 2019
medline: 26 2 2019
Statut: epublish

Résumé

The advancement of nanofluidic applications will require the identification of materials with high-conductivity nanoscale channels that can be readily obtained at massive scale. Inspired by the transpiration in mesostructured trees, we report a nanofluidic membrane consisting of densely packed cellulose nanofibers directly derived from wood. Numerous nanochannels are produced among an expansive array of one-dimensional cellulose nanofibers. The abundant functional groups of cellulose enable facile tuning of the surface charge density via chemical modification. The nanofiber-nanofiber spacing can also be tuned from ~2 to ~20 nm by structural engineering. The surface-charge-governed ionic transport region shows a high ionic conductivity plateau of ~2 mS cm

Identifiants

pubmed: 30801009
doi: 10.1126/sciadv.aau4238
pii: aau4238
pmc: PMC6386557
doi:

Types de publication

Journal Article

Langues

eng

Pagination

eaau4238

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Auteurs

Tian Li (T)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Sylvia Xin Li (SX)

Department of Physics, Yale University, New Haven, CT 06511, USA.

Weiqing Kong (W)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Chaoji Chen (C)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Emily Hitz (E)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Chao Jia (C)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Jiaqi Dai (J)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Xin Zhang (X)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Robert Briber (R)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Zuzanna Siwy (Z)

Department of Physics and Astronomy, University of California, Irvine, Irvine, CA 92697, USA.

Mark Reed (M)

Departments of Electrical Engineering and Applied Physics, Yale University, New Haven, CT 06520, USA.

Liangbing Hu (L)

Department of Materials Science and Engineering, University of Maryland College Park, College Park, MD 20742, USA.

Classifications MeSH