CD44 targeted delivery of siRNA by using HA-decorated nanotechnologies for KRAS silencing in cancer treatment.


Journal

International journal of pharmaceutics
ISSN: 1873-3476
Titre abrégé: Int J Pharm
Pays: Netherlands
ID NLM: 7804127

Informations de publication

Date de publication:
20 Apr 2019
Historique:
received: 11 12 2018
revised: 21 01 2019
accepted: 18 02 2019
pubmed: 2 3 2019
medline: 20 8 2019
entrez: 2 3 2019
Statut: ppublish

Résumé

KRAS is a small GTPase that regulates cell proliferation and survival. In tumors, the KRAS gene is mutated, and leading to unregulated tumor growth. Despite the recognized importance of KRAS in cancer, attempts to develop small molecule inhibitors have proved unsuccessful. An alternative strategy is gene silencing and the use of small nucleic acid sequences (e.g. siRNA, shRNA), has been reported to successfully downregulate KRAS. In this study we developed ternary nanocomplexes to deliver an anti-KRAS siRNA to colorectal cancer cells, exploiting the interaction of hyaluronic acid (HA) with CD44 as a means to achieve selective targeting of CD44-positive cancer cells. Two different polycations, poly(hexamethylene biguanide) and chitosan, were complexed with siRNA and coated with HA. Physico-chemical properties and stability of nanoparticles were characterized, including size, surface charge, and degree of siRNA protection. We demonstrate nanoparticle internalization (flow cytometry), siRNA cytosolic release (confocal microscopy) and KRAS silencing (RT-qPCR) in CD44

Identifiants

pubmed: 30822503
pii: S0378-5173(19)30155-3
doi: 10.1016/j.ijpharm.2019.02.032
pii:
doi:

Substances chimiques

Biguanides 0
Hyaluronan Receptors 0
KRAS protein, human 0
RNA, Small Interfering 0
polihexanide 322U039GMF
Hyaluronic Acid 9004-61-9
Chitosan 9012-76-4
Proto-Oncogene Proteins p21(ras) EC 3.6.5.2

Types de publication

Journal Article

Langues

eng

Pagination

114-123

Informations de copyright

Copyright © 2019 Elsevier B.V. All rights reserved.

Auteurs

A Tirella (A)

Division of Pharmacy and Optometry, Faculty of Biology, Medicine and Health, University of Manchester, Manchester Academic Health Science Centre, Oxford Road, Manchester M13 9PL, United Kingdom; NorthWest Centre for Advanced Drug Delivery (NoWCADD), Faculty of Biology, Medicine and Health, University of Manchester, Oxford Road, Manchester M13 9PT, United Kingdom. Electronic address: annalisa.tirella@manchester.ac.uk.

K Kloc-Muniak (K)

Tecrea Ltd. 2 Royal College Street, London NW1 0NH, United Kingdom.

L Good (L)

Tecrea Ltd. 2 Royal College Street, London NW1 0NH, United Kingdom; Department of Pathology and Population Sciences, Royal Veterinary College, Royal College Street, London NW1 0TU, United Kingdom.

J Ridden (J)

Tecrea Ltd. 2 Royal College Street, London NW1 0NH, United Kingdom.

M Ashford (M)

Advanced Drug Delivery, Pharmaceutical Sciences, IMED Biotech Unit, AstraZeneca, Cambridge, United Kingdom.

S Puri (S)

Advanced Drug Delivery, Pharmaceutical Sciences, IMED Biotech Unit, AstraZeneca, Cambridge, United Kingdom.

N Tirelli (N)

Division of Pharmacy and Optometry, Faculty of Biology, Medicine and Health, University of Manchester, Manchester Academic Health Science Centre, Oxford Road, Manchester M13 9PL, United Kingdom; NorthWest Centre for Advanced Drug Delivery (NoWCADD), Faculty of Biology, Medicine and Health, University of Manchester, Oxford Road, Manchester M13 9PT, United Kingdom; Laboratory of Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy.

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Classifications MeSH