Out-of-equilibrium electron dynamics of silver driven by ultrafast electromagnetic fields - a novel hydrodynamical approach.


Journal

Faraday discussions
ISSN: 1364-5498
Titre abrégé: Faraday Discuss
Pays: England
ID NLM: 9212301

Informations de publication

Date de publication:
23 05 2019
Historique:
pubmed: 7 3 2019
medline: 7 3 2019
entrez: 7 3 2019
Statut: ppublish

Résumé

We investigate the ultrafast nonlinear response of silver upon excitation by infrared electromagnetic radiation pulses with a duration of a few femtoseconds. By adopting the Landau weak coupling approach to account for electron-electron and electron-phonon collisions, we solve the Boltzmann equation through the method of moments obtaining a novel set of hydrodynamical equations describing the ultrafast nonlinear dynamics of electrons in silver. While the novel hydrodynamical model that was obtained reduces to the Drude model for small intensities of the driving field, it predicts that absorption saturates for large but experimentally attainable peak intensities of the order of GW cm-2. Our results are important for absorption mitigation in plasmonic devices, with potential impact for low-loss plasmonic waveguides and interconnects.

Identifiants

pubmed: 30838372
doi: 10.1039/c8fd00153g
doi:

Types de publication

Journal Article Research Support, U.S. Gov't, Non-P.H.S. Research Support, Non-U.S. Gov't

Langues

eng

Pagination

235-243

Auteurs

Andrea Marini (A)

Department of Physical and Chemical Sciences, University of L'Aquila, Via Vetoio, 67100 L'Aquila, Italy. andrea.marini@aquila.infn.it.

Classifications MeSH