Chitosan functionalization of titanium and Ti6Al4V alloy with chloroacetic acid as linker agent.


Journal

Materials science & engineering. C, Materials for biological applications
ISSN: 1873-0191
Titre abrégé: Mater Sci Eng C Mater Biol Appl
Pays: Netherlands
ID NLM: 101484109

Informations de publication

Date de publication:
Jun 2019
Historique:
received: 26 07 2018
revised: 25 01 2019
accepted: 15 02 2019
entrez: 21 3 2019
pubmed: 21 3 2019
medline: 12 7 2019
Statut: ppublish

Résumé

In this work, a new covalent grafting of chitosan on titanium and Ti6Al4V alloy surfaces is reported using chloroacetic acid as linker agent. Good results were obtained both on titanium and on Ti6Al4V alloy. The effect of the surface acid pretreatments on the subsequent functionalization with chitosan is evaluated. The morphological aspect of acid etched metal surfaces before chitosan grafting has been characterized by scanning electron microscopy (SEM). The presence of carboxylic groups on metal surfaces and then the efficiency of chitosan covalent immobilization were detected by Fourier transformed infrared-Attenuated Total Reflectance (FTIR-ATR) and X-Ray photoelectron spectroscopy (XPS). Cyclic voltammetry tests, using the functionalized titanium and Ti6Al4V samples as electrodes, were conducted in different aqueous solutions, to detect the presence of the homogeneous overlayer of chitosan on the surface, and to evaluate the importance of the carboxyl groups as linker agent.

Identifiants

pubmed: 30889647
pii: S0928-4931(18)32214-8
doi: 10.1016/j.msec.2019.02.052
pii:
doi:

Substances chimiques

Acetates 0
Alloys 0
titanium alloy (TiAl6V4) 12743-70-3
chloroacetic acid 5GD84Y125G
Chitosan 9012-76-4
Titanium D1JT611TNE

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

1133-1140

Informations de copyright

Copyright © 2019 Elsevier B.V. All rights reserved.

Auteurs

Chiara Battocchio (C)

Department of Science, Roma Tre University, Via della Vasca navale 79, Roma, Italy.

Sofia Concolato (S)

Department of Engineering, Roma Tre University, via Vito Volterra 62, Roma, Italy.

Serena De Santis (S)

Department of Engineering, Roma Tre University, via Vito Volterra 62, Roma, Italy.

Mats Fahlman (M)

Division of Surface Physics and Chemistry, IFM, Linkoping University, Linkoping, Sweden.

Giovanna Iucci (G)

Department of Science, Roma Tre University, Via della Vasca navale 79, Roma, Italy.

Marta Santi (M)

Department of Science, Roma Tre University, Via della Vasca navale 79, Roma, Italy.

Giovanni Sotgiu (G)

Department of Engineering, Roma Tre University, via Vito Volterra 62, Roma, Italy.

Monica Orsini (M)

Department of Engineering, Roma Tre University, via Vito Volterra 62, Roma, Italy. Electronic address: monica.orsini@uniroma3.it.

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Classifications MeSH