Motion of active tracer in a lattice gas with cross-shaped particles.


Journal

The Journal of chemical physics
ISSN: 1089-7690
Titre abrégé: J Chem Phys
Pays: United States
ID NLM: 0375360

Informations de publication

Date de publication:
14 Apr 2019
Historique:
entrez: 15 4 2019
pubmed: 15 4 2019
medline: 15 4 2019
Statut: ppublish

Résumé

We analyze the dynamics of an active tracer particle embedded in a thermal lattice gas. All particles are subject to exclusion up to third nearest neighbors on the square lattice, which leads to slow dynamics at high densities. For the case with no rotational diffusion of the tracer, we derive an analytical expression for the resulting drift velocity v of the tracer in terms of non-equilibrium density correlations involving the tracer particle and its neighbors, which we verify using numerical simulations. We show that the properties of the passive system alone do not adequately describe even this simple system of a single non-rotating active tracer. For large activity and low density, we develop an approximation for v. For the case where the tracer undergoes rotational diffusion independent of its neighbors, we relate its diffusion coefficient to the thermal diffusion coefficient and v. Finally, we study dynamics where the rotation of the tracer is limited by the presence of neighboring particles. We find that the effect of this rotational locking may be quantitatively described in terms of a reduction in the rotation rate.

Identifiants

pubmed: 30981244
doi: 10.1063/1.5085769
doi:

Types de publication

Journal Article

Langues

eng

Pagination

144508

Auteurs

Rakesh Chatterjee (R)

School of Mechanical Engineering and Sackler Center for Computational Molecular and Materials Science, Tel Aviv University, Tel Aviv 69978, Israel.

Nimrod Segall (N)

School of Mechanical Engineering and Sackler Center for Computational Molecular and Materials Science, Tel Aviv University, Tel Aviv 69978, Israel.

Carl Merrigan (C)

Martin Fisher School of Physics, Brandeis University, Waltham, Massachusetts 02454, USA.

Kabir Ramola (K)

Martin Fisher School of Physics, Brandeis University, Waltham, Massachusetts 02454, USA.

Bulbul Chakraborty (B)

Martin Fisher School of Physics, Brandeis University, Waltham, Massachusetts 02454, USA.

Yair Shokef (Y)

School of Mechanical Engineering and Sackler Center for Computational Molecular and Materials Science, Tel Aviv University, Tel Aviv 69978, Israel.

Classifications MeSH