Dynamic Nuclear Polarization / solid-state NMR of membranes. Thermal effects and sample geometry.


Journal

Solid state nuclear magnetic resonance
ISSN: 1527-3326
Titre abrégé: Solid State Nucl Magn Reson
Pays: Netherlands
ID NLM: 9306181

Informations de publication

Date de publication:
08 2019
Historique:
received: 27 12 2018
revised: 18 03 2019
accepted: 18 03 2019
pubmed: 18 4 2019
medline: 18 4 2019
entrez: 18 4 2019
Statut: ppublish

Résumé

Whereas specially designed dinitroxide biradicals, reconstitution protocols, oriented sample geometries and NMR probes have helped to much increase the DNP enhancement factors of membrane samples they still lag considerably behind those obtained from glasses made of protein solutions. Here we show that not only the MAS rotor material but also the distribution of the membrane samples within the NMR rotor have a pronounced effect on the DNP enhancement. These observations are rationalized with the cooling efficiency and the internal properties of the sample, monitored by their T

Identifiants

pubmed: 30995597
pii: S0926-2040(18)30113-9
doi: 10.1016/j.ssnmr.2019.03.004
pii:
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

70-76

Informations de copyright

Copyright © 2019. Published by Elsevier Inc.

Auteurs

Evgeniy Sergeevich Salnikov (ES)

Institute of Chemistry, University of Strasbourg / CNRS, UMR7177, 67070, Strasbourg, France.

Fabien Aussenac (F)

Bruker BioSpin, Wissembourg, France.

Sebastian Abel (S)

Aix-Marseille University, CNRS, UMR 7273, Institut de Chimie Radicalaire, 13013, Marseille, France.

Armin Purea (A)

Bruker BioSpin, Rheinstetten, Germany.

Paul Tordo (P)

Aix-Marseille University, CNRS, UMR 7273, Institut de Chimie Radicalaire, 13013, Marseille, France.

Olivier Ouari (O)

Aix-Marseille University, CNRS, UMR 7273, Institut de Chimie Radicalaire, 13013, Marseille, France.

Burkhard Bechinger (B)

Institute of Chemistry, University of Strasbourg / CNRS, UMR7177, 67070, Strasbourg, France. Electronic address: bechinge@unistra.fr.

Classifications MeSH