Metal-organic framework (MOF-5) coated SERS active gold gratings: A platform for the selective detection of organic contaminants in soil.

Gold grating Metal-organic framework Organophosphorus pesticides Reproducibility SERS Selectivity Soil sample Surface-assisted MOF growth

Journal

Analytica chimica acta
ISSN: 1873-4324
Titre abrégé: Anal Chim Acta
Pays: Netherlands
ID NLM: 0370534

Informations de publication

Date de publication:
30 Aug 2019
Historique:
received: 30 01 2019
revised: 22 03 2019
accepted: 28 03 2019
entrez: 11 5 2019
pubmed: 11 5 2019
medline: 11 5 2019
Statut: ppublish

Résumé

In this work, we proposed the functionalization of a surface plasmon-polariton (SPP)-supported gold grating surface with the metal-organic framework (MOF-5) for sensitive, selective and reproducible surface-enhanced Raman scattering (SERS) detection of organophosphorus pesticides. Homogeneous distribution of plasmon intensity along the Au grating surface ensures the high reproducibility of SERS results (deviation of Raman peak intensity does not exceed the 4% along the sample). The surface-assisted growth of thin MOF-5 film was accomplished in two steps procedure: (i) covalent grafting by 4-carboxyphenyl groups and (ii) the immersion of samples in the mother liquid of MOF-5. Proposed SERS chip proved itself to be a perfect analytical probe for the detection of organophosphorus pesticides with high reliability and low detection limit up to 10

Identifiants

pubmed: 31072479
pii: S0003-2670(19)30376-9
doi: 10.1016/j.aca.2019.03.058
pii:
doi:

Types de publication

Journal Article

Langues

eng

Pagination

70-79

Informations de copyright

Copyright © 2019 Elsevier B.V. All rights reserved.

Auteurs

O Guselnikova (O)

Department of Solid State Engineering, University of Chemistry and Technology, 16628, Prague, Czech Republic; Research School of Chemistry and Applied Biomedical Sciences, Tomsk Polytechnic University, Russian Federation.

P Postnikov (P)

Department of Solid State Engineering, University of Chemistry and Technology, 16628, Prague, Czech Republic; Research School of Chemistry and Applied Biomedical Sciences, Tomsk Polytechnic University, Russian Federation. Electronic address: postnikov@tpu.ru.

R Elashnikov (R)

Research School of Chemistry and Applied Biomedical Sciences, Tomsk Polytechnic University, Russian Federation.

E Miliutina (E)

Department of Solid State Engineering, University of Chemistry and Technology, 16628, Prague, Czech Republic; Research School of Chemistry and Applied Biomedical Sciences, Tomsk Polytechnic University, Russian Federation.

V Svorcik (V)

Research School of Chemistry and Applied Biomedical Sciences, Tomsk Polytechnic University, Russian Federation.

O Lyutakov (O)

Department of Solid State Engineering, University of Chemistry and Technology, 16628, Prague, Czech Republic; Research School of Chemistry and Applied Biomedical Sciences, Tomsk Polytechnic University, Russian Federation. Electronic address: lyutakoo@vscht.cz.

Classifications MeSH