Possible observation of quantum spin-nematic phase in a frustrated magnet.
calorimetry
hidden order
high magnetic field
magnetism
spin nematic
Journal
Proceedings of the National Academy of Sciences of the United States of America
ISSN: 1091-6490
Titre abrégé: Proc Natl Acad Sci U S A
Pays: United States
ID NLM: 7505876
Informations de publication
Date de publication:
28 May 2019
28 May 2019
Historique:
pubmed:
11
5
2019
medline:
11
5
2019
entrez:
11
5
2019
Statut:
ppublish
Résumé
Water freezes into ice in winter and evaporates into vapor in summer. Scientifically, the transformations between solid, liquid, and gas are called phase transitions and can be classified through the changes in symmetry which occur in each case. A fourth phase of matter was discovered late in the 19th century: the liquid crystal nematic, in which rod- or disk-shaped molecules align like the atoms in a solid, while continuing to flow like a liquid. Here we report thermodynamic evidence of a quantum analog of the classical nematic phase, the quantum spin nematic (SN). In an SN, the spins of a quantum magnet select a common axis, like a nematic liquid crystal, while escaping conventional magnetic order. Our state-of-the-art thermal measurements in high pulsed magnetic fields up to 33 T on the copper mineral volborthite with spin 1/2 on a frustrated lattice provide thermodynamic evidence for SN order, half a century after the theoretical proposal [Blume M, Hsieh YY (1969)
Identifiants
pubmed: 31072923
pii: 1821969116
doi: 10.1073/pnas.1821969116
pmc: PMC6561203
doi:
Types de publication
Journal Article
Langues
eng
Pagination
10686-10690Informations de copyright
Copyright © 2019 the Author(s). Published by PNAS.
Déclaration de conflit d'intérêts
The authors declare no conflict of interest.
Références
Phys Rev Lett. 2015 Jun 5;114(22):227202
pubmed: 26196641
Phys Rev Lett. 2017 Jun 16;118(24):247201
pubmed: 28665634
Phys Rev Lett. 2016 Jul 15;117(3):037206
pubmed: 27472136
Phys Rev Lett. 2006 Jan 20;96(2):027213
pubmed: 16486634
Sci Rep. 2019 Oct 8;9(1):14468
pubmed: 31594985
Acta Crystallogr C. 2012 Jul;68(Pt 7):i41-4
pubmed: 22763677
Nat Commun. 2012 May 29;3:860
pubmed: 22643887
Science. 2009 Sep 11;325(5946):1360-3
pubmed: 19661381
Phys Rev B Condens Matter. 1991 Sep 1;44(9):4693-4696
pubmed: 10000135