The role of soil components in synthetic mixtures during the adsorption and speciation changes of Cr(VI): Conjunction of the modeling approach with spectroscopic and isotopic investigations.


Journal

Environment international
ISSN: 1873-6750
Titre abrégé: Environ Int
Pays: Netherlands
ID NLM: 7807270

Informations de publication

Date de publication:
06 2019
Historique:
received: 30 11 2018
revised: 26 02 2019
accepted: 27 03 2019
pubmed: 11 5 2019
medline: 23 10 2019
entrez: 11 5 2019
Statut: ppublish

Résumé

This study investigates redox transitions associated with the adsorption of Cr(VI) on commonly occurring soil components (silicates, oxides and humic acids) and their synthetic mixtures by coupling the mechanistic surface complexation modeling with spectroscopic and isotopic analyses. The mixtures of soil components were prepared to reflect the composition of the real anthroposol sample, determined by X-ray Powder Diffraction (XRD), total organic carbon (TOC) measurement and extraction methods. The effect of different initial Cr(VI) concentrations (2×10

Identifiants

pubmed: 31075676
pii: S0160-4120(18)32943-X
doi: 10.1016/j.envint.2019.03.066
pii:
doi:

Substances chimiques

Ferric Compounds 0
Soil 0
Soil Pollutants 0
Chromium 0R0008Q3JB
chromium hexavalent ion 18540-29-9
ferric oxide 1K09F3G675
ferric oxyhydroxide 87PZU03K0K

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

848-857

Informations de copyright

Copyright © 2019 The Authors. Published by Elsevier Ltd.. All rights reserved.

Auteurs

Veronika Veselská (V)

Department of Environmental Geosciences, Faculty of Environmental Sciences, Czech University of Life Sciences Prague, Kamýcká 129, CZ-16500 Prague, Czech Republic. Electronic address: veselskav@fzp.czu.cz.

Hana Šillerová (H)

Department of Environmental Geosciences, Faculty of Environmental Sciences, Czech University of Life Sciences Prague, Kamýcká 129, CZ-16500 Prague, Czech Republic.

Jörg Göttlicher (J)

Institute for Photon Science and Synchrotron Radiation, Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz 1, DE-76344 Eggenstein-Leopoldshafen, Germany.

Zuzana Michálková (Z)

Department of Environmental Geosciences, Faculty of Environmental Sciences, Czech University of Life Sciences Prague, Kamýcká 129, CZ-16500 Prague, Czech Republic.

Jamal A Siddique (JA)

Department of Environmental Geosciences, Faculty of Environmental Sciences, Czech University of Life Sciences Prague, Kamýcká 129, CZ-16500 Prague, Czech Republic.

Sylva Číhalová (S)

Department of Environmental Geosciences, Faculty of Environmental Sciences, Czech University of Life Sciences Prague, Kamýcká 129, CZ-16500 Prague, Czech Republic.

Vladislav Chrastný (V)

Department of Environmental Geosciences, Faculty of Environmental Sciences, Czech University of Life Sciences Prague, Kamýcká 129, CZ-16500 Prague, Czech Republic.

Ralph Steininger (R)

Institute for Photon Science and Synchrotron Radiation, Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz 1, DE-76344 Eggenstein-Leopoldshafen, Germany.

Stefan Mangold (S)

Institute for Photon Science and Synchrotron Radiation, Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz 1, DE-76344 Eggenstein-Leopoldshafen, Germany.

Michael Komárek (M)

Department of Environmental Geosciences, Faculty of Environmental Sciences, Czech University of Life Sciences Prague, Kamýcká 129, CZ-16500 Prague, Czech Republic.

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