Quercetin-3-oleoyl derivatives as new GPR40 agonists: Molecular docking studies and functional evaluation.

GPR40 allosteric site Insulin secretion Oleic acid Quercetin Type 2 diabetes

Journal

Bioorganic & medicinal chemistry letters
ISSN: 1464-3405
Titre abrégé: Bioorg Med Chem Lett
Pays: England
ID NLM: 9107377

Informations de publication

Date de publication:
15 07 2019
Historique:
received: 15 02 2019
revised: 07 05 2019
accepted: 11 05 2019
pubmed: 21 5 2019
medline: 10 9 2020
entrez: 21 5 2019
Statut: ppublish

Résumé

The G-protein-coupled receptor 40 (GPR40) is an attractive molecular target for the treatment of type 2 diabetes mellitus. Previously, based on the natural oleic acid substrate, an exogenous ligand for this receptor, named AV1, was synthesized. In this context, here we validated the activity of AV1 as a full agonist, while the corresponding catechol analogue, named AV2, was investigated for the first time. The ligand-protein interaction between this new molecule and the receptor was highlighted in the lower portion of the GPR40 groove that generally accommodates DC260126. The functional assays performed have demonstrated that AV2 is a suitable GPR40 partial agonist, showing a therapeutic potential and representing a useful tool in the management of type 2 diabetes.

Identifiants

pubmed: 31104992
pii: S0960-894X(19)30315-4
doi: 10.1016/j.bmcl.2019.05.018
pii:
doi:

Substances chimiques

Quercetin 9IKM0I5T1E

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1761-1764

Informations de copyright

Copyright © 2019 Elsevier Ltd. All rights reserved.

Auteurs

Gabriele Carullo (G)

Department of Pharmacy, Health and Nutritional Sciences, "Dipartimento di Eccellenza 2018-2022", University of Calabria, Edificio Polifunzionale, 87036 Rende, Italy.

Mariarita Perri (M)

Department of Pharmacy, Health and Nutritional Sciences, "Dipartimento di Eccellenza 2018-2022", University of Calabria, Edificio Polifunzionale, 87036 Rende, Italy.

Fabrizio Manetti (F)

Department of Biotechnology, Chemistry and Pharmacy, "Dipartimento di Eccellenza 2018-2022", University of Siena, Via Aldo Moro, 2, 53100 Siena, Italy.

Francesca Aiello (F)

Department of Pharmacy, Health and Nutritional Sciences, "Dipartimento di Eccellenza 2018-2022", University of Calabria, Edificio Polifunzionale, 87036 Rende, Italy. Electronic address: francesca.aiello@unical.it.

Maria Cristina Caroleo (MC)

Department of Pharmacy, Health and Nutritional Sciences, "Dipartimento di Eccellenza 2018-2022", University of Calabria, Edificio Polifunzionale, 87036 Rende, Italy.

Erika Cione (E)

Department of Pharmacy, Health and Nutritional Sciences, "Dipartimento di Eccellenza 2018-2022", University of Calabria, Edificio Polifunzionale, 87036 Rende, Italy.

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Classifications MeSH