A Metal-Organic Framework Based Methane Nano-trap for the Capture of Coal-Mine Methane.

coal-mine methane cooperative effect gas separation metal-organic frameworks nano-traps

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
22 Jul 2019
Historique:
received: 11 04 2019
pubmed: 23 5 2019
medline: 23 5 2019
entrez: 23 5 2019
Statut: ppublish

Résumé

As a major greenhouse gas, methane, which is directly vented from the coal-mine to the atmosphere, has not yet drawn sufficient attention. To address this problem, we report a methane nano-trap that features oppositely adjacent open metal sites and dense alkyl groups in a metal-organic framework (MOF). The alkyl MOF-based methane nano-trap exhibits a record-high methane uptake and CH

Identifiants

DOI: 10.1002/anie.201904507 PMID: 31115966
pubmed: 31115966
doi: 10.1002/anie.201904507
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

10138-10141

Subventions

Organisme : Division of Materials Research
ID : DMR-1352065
Organisme : Division of Materials Research
ID : DMR-1607989
Organisme : Division of Chemistry
ID : CHE-1531590
Organisme : American Chemical Society Petroleum Research Fund
ID : 56673-ND6

Informations de copyright

© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Auteurs

Zheng Niu (Z)

Department of Chemistry, University of South Florida, 4202 E. Fowler Avenue, Tampa, FL, 33620, USA.

Xili Cui (X)

Department of Chemistry, University of South Florida, 4202 E. Fowler Avenue, Tampa, FL, 33620, USA.
Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, 310027, China.

Tony Pham (T)

Department of Chemistry, University of South Florida, 4202 E. Fowler Avenue, Tampa, FL, 33620, USA.

Pui Ching Lan (PC)

Department of Chemistry, University of South Florida, 4202 E. Fowler Avenue, Tampa, FL, 33620, USA.

Huabin Xing (H)

Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, 310027, China.

Katherine A Forrest (KA)

Department of Chemistry, University of South Florida, 4202 E. Fowler Avenue, Tampa, FL, 33620, USA.

Lukasz Wojtas (L)

Department of Chemistry, University of South Florida, 4202 E. Fowler Avenue, Tampa, FL, 33620, USA.

Brian Space (B)

Department of Chemistry, University of South Florida, 4202 E. Fowler Avenue, Tampa, FL, 33620, USA.

Shengqian Ma (S)

Department of Chemistry, University of South Florida, 4202 E. Fowler Avenue, Tampa, FL, 33620, USA.
ORCID: 0000-0002-1897-7069

Classifications MeSH