Oxidative Coupling of Terminal Rhenium Pnictide Complexes.

QTAIM dipnictides pincer complexes pnictides rhenium

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
05 Aug 2019
Historique:
received: 24 04 2019
revised: 27 05 2019
pubmed: 11 6 2019
medline: 11 6 2019
entrez: 11 6 2019
Statut: ppublish

Résumé

The isolation of rhenium(V) complexes with terminal phosphide and arsenide ligands was achieved upon decarbonylation of rhenium(III) pnictaethynolates. One-electron oxidation of the pnictide complexes yielded Pn-Pn (Pn=P, As) coupling products, which were spectroscopically and crystallographically characterized. Computational bond analysis suggests that these complexes are best described as {Pn

Identifiants

pubmed: 31179626
doi: 10.1002/anie.201905130
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

10966-10970

Subventions

Organisme : European Research Council
ID : CoG 646747
Pays : International
Organisme : Fonds der Chemischen Industrie

Informations de copyright

© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Auteurs

Josh Abbenseth (J)

Georg-August-Universität, Institut für Anorganische Chemie, Tammannstraße 4, 37077, Göttingen, Germany.

Martin Diefenbach (M)

Institut für Anorganische und Analytische Chemie, Goethe-Universität, Max-von-Laue-Strasse 7, 60438, Frankfurt am Main, Germany.

Alexander Hinz (A)

Karlsruhe Institute of Technology, Institute of Inorganic Chemistry, Engesserstr. 15, 76131, Karlsruhe, Germany.

Lukas Alig (L)

Georg-August-Universität, Institut für Anorganische Chemie, Tammannstraße 4, 37077, Göttingen, Germany.

Christian Würtele (C)

Georg-August-Universität, Institut für Anorganische Chemie, Tammannstraße 4, 37077, Göttingen, Germany.

Jose M Goicoechea (JM)

Department of Chemistry, University of Oxford, Chemistry Research Laboratory, 12 Mansfield Road, OX1 3TA, Oxford, UK.

Max C Holthausen (MC)

Institut für Anorganische und Analytische Chemie, Goethe-Universität, Max-von-Laue-Strasse 7, 60438, Frankfurt am Main, Germany.

Sven Schneider (S)

Georg-August-Universität, Institut für Anorganische Chemie, Tammannstraße 4, 37077, Göttingen, Germany.

Classifications MeSH