A universal approach for the synthesis of two-dimensional binary compounds.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
04 Jul 2019
Historique:
received: 07 01 2019
accepted: 20 06 2019
entrez: 6 7 2019
pubmed: 6 7 2019
medline: 6 7 2019
Statut: epublish

Résumé

Only a few of the vast range of potential two-dimensional materials (2D) have been isolated or synthesised to date. Typically, 2D materials are discovered by mechanically exfoliating naturally occurring bulk crystals to produce atomically thin layers, after which a material-specific vapour synthesis method must be developed to grow interesting candidates in a scalable manner. Here we show a general approach for synthesising thin layers of two-dimensional binary compounds. We apply the method to obtain high quality, epitaxial MoS

Identifiants

pubmed: 31273207
doi: 10.1038/s41467-019-11075-2
pii: 10.1038/s41467-019-11075-2
pmc: PMC6609655
doi:

Types de publication

Journal Article

Langues

eng

Pagination

2957

Subventions

Organisme : EC | EU Framework Programme for Research and Innovation H2020 | H2020 Priority Excellent Science | H2020 Future and Emerging Technologies (H2020 Excellent Science - Future and Emerging Technologies)
ID : 785219
Organisme : EC | EU Framework Programme for Research and Innovation H2020 | H2020 Priority Excellent Science | H2020 Future and Emerging Technologies (H2020 Excellent Science - Future and Emerging Technologies)
ID : 696656
Organisme : EC | EU Framework Programme for Research and Innovation H2020 | H2020 Priority Excellent Science | H2020 Future and Emerging Technologies (H2020 Excellent Science - Future and Emerging Technologies)
ID : 785219
Organisme : EC | Seventh Framework Programme (EC Seventh Framework Programm)
ID : FP7-6040007
Organisme : Danmarks Grundforskningsfond (Danish National Research Foundation)
ID : DNRF103
Organisme : Danmarks Grundforskningsfond (Danish National Research Foundation)
ID : DNRF122
Organisme : Villum Fonden (Villum Foundation)
ID : 11744
Organisme : Villum Fonden (Villum Foundation)
ID : 9455
Organisme : Villum Fonden (Villum Foundation)
ID : 9301

Références

ACS Nano. 2014 May 27;8(5):5125-31
pubmed: 24680389
ACS Nano. 2014 Oct 28;8(10):10196-204
pubmed: 25211696
Science. 2018 Nov 16;362(6416):817-821
pubmed: 30442807
Nat Commun. 2017 Oct 16;8(1):958
pubmed: 29038430
Nature. 2018 Apr;556(7701):355-359
pubmed: 29670263
Ultramicroscopy. 2015 Apr;151:62-67
pubmed: 25465498
Proc Natl Acad Sci U S A. 2016 Oct 18;113(42):11688-11693
pubmed: 27092006
ACS Nano. 2013 Jun 25;7(6):5235-42
pubmed: 23647141
Nature. 2015 Apr 30;520(7549):656-60
pubmed: 25925478
Nat Commun. 2015 Oct 09;6:8569
pubmed: 26450174
Nat Nanotechnol. 2014 Feb;9(2):111-5
pubmed: 24362235
Nature. 2013 Jul 25;499(7459):419-25
pubmed: 23887427
ACS Nano. 2015 Apr 28;9(4):3596-604
pubmed: 25785299
Angew Chem Int Ed Engl. 2014 Jan 27;53(5):1266-9
pubmed: 24420501
Nanoscale. 2012 Oct 21;4(20):6637-41
pubmed: 22983609
ACS Nano. 2013 Apr 23;7(4):2898-926
pubmed: 23464873
Chem Mater. 2014 Nov 25;26(22):6380-6392
pubmed: 25673919
ACS Appl Mater Interfaces. 2018 Nov 28;10(47):40831-40837
pubmed: 30384598
Nat Commun. 2016 Dec 20;7:13911
pubmed: 27996005
ACS Nano. 2015 Jun 23;9(6):6502-10
pubmed: 26039108
Nano Lett. 2010 May 12;10(5):1912-6
pubmed: 20402493
ACS Nano. 2015 May 26;9(5):5510-9
pubmed: 25873415
Nat Mater. 2015 Nov;14(11):1135-41
pubmed: 26280223
Adv Mater. 2012 May 2;24(17):2320-5
pubmed: 22467187
Chem Soc Rev. 2015 May 7;44(9):2744-56
pubmed: 25327436
Langmuir. 2015 Sep 8;31(35):9700-6
pubmed: 26308879
Chem Rev. 2017 May 10;117(9):6225-6331
pubmed: 28306244
Chem Soc Rev. 2014 Sep 21;43(18):6537-54
pubmed: 24825454
Nat Commun. 2015 Oct 15;6:8563
pubmed: 26469634
Science. 2009 Jun 5;324(5932):1312-4
pubmed: 19423775

Auteurs

Abhay Shivayogimath (A)

DTU Physics, Technical University of Denmark, Ørsteds Plads 345, DK-2800 Kgs, Lyngby, Denmark.
Centre for Nanostructured Graphene (CNG), Technical University of Denmark, Ørsteds Plads 345C, DK-2800 Kgs, Lyngby, Denmark.

Joachim Dahl Thomsen (JD)

DTU Physics, Technical University of Denmark, Ørsteds Plads 345, DK-2800 Kgs, Lyngby, Denmark.
Centre for Nanostructured Graphene (CNG), Technical University of Denmark, Ørsteds Plads 345C, DK-2800 Kgs, Lyngby, Denmark.

David M A Mackenzie (DMA)

Centre for Nanostructured Graphene (CNG), Technical University of Denmark, Ørsteds Plads 345C, DK-2800 Kgs, Lyngby, Denmark.
Department of Electronics and Nanoengineering, Aalto University, P.O. Box 13500, FI-00076, Aalto, Finland.

Mathias Geisler (M)

Centre for Nanostructured Graphene (CNG), Technical University of Denmark, Ørsteds Plads 345C, DK-2800 Kgs, Lyngby, Denmark.
DTU Fotonik, Technical University of Denmark, Ørsteds Plads 343, DK-2800 Kgs, Lyngby, Denmark.

Raluca-Maria Stan (RM)

Department of Physics and Astronomy, Interdisciplinary Nanoscience Center (iNANO), Aarhus University, 8000, Aarhus, Denmark.

Ann Julie Holt (AJ)

Department of Physics and Astronomy, Interdisciplinary Nanoscience Center (iNANO), Aarhus University, 8000, Aarhus, Denmark.

Marco Bianchi (M)

Department of Physics and Astronomy, Interdisciplinary Nanoscience Center (iNANO), Aarhus University, 8000, Aarhus, Denmark.

Andrea Crovetto (A)

DTU Physics, Technical University of Denmark, Fysikvej 312, DK-2800 Kgs, Lyngby, Denmark.

Patrick R Whelan (PR)

DTU Physics, Technical University of Denmark, Ørsteds Plads 345, DK-2800 Kgs, Lyngby, Denmark.
Centre for Nanostructured Graphene (CNG), Technical University of Denmark, Ørsteds Plads 345C, DK-2800 Kgs, Lyngby, Denmark.

Alexandra Carvalho (A)

Centre for Advanced 2D Materials and Graphene Research Centre, National University of Singapore, 2 Science Drive 3, Singapore, 117542, Singapore.

Antonio H Castro Neto (AHC)

Centre for Advanced 2D Materials and Graphene Research Centre, National University of Singapore, 2 Science Drive 3, Singapore, 117542, Singapore.

Philip Hofmann (P)

Department of Physics and Astronomy, Interdisciplinary Nanoscience Center (iNANO), Aarhus University, 8000, Aarhus, Denmark.

Nicolas Stenger (N)

Centre for Nanostructured Graphene (CNG), Technical University of Denmark, Ørsteds Plads 345C, DK-2800 Kgs, Lyngby, Denmark.
DTU Fotonik, Technical University of Denmark, Ørsteds Plads 343, DK-2800 Kgs, Lyngby, Denmark.

Peter Bøggild (P)

DTU Physics, Technical University of Denmark, Ørsteds Plads 345, DK-2800 Kgs, Lyngby, Denmark.
Centre for Nanostructured Graphene (CNG), Technical University of Denmark, Ørsteds Plads 345C, DK-2800 Kgs, Lyngby, Denmark.

Timothy J Booth (TJ)

DTU Physics, Technical University of Denmark, Ørsteds Plads 345, DK-2800 Kgs, Lyngby, Denmark. tibo@dtu.dk.
Centre for Nanostructured Graphene (CNG), Technical University of Denmark, Ørsteds Plads 345C, DK-2800 Kgs, Lyngby, Denmark. tibo@dtu.dk.

Classifications MeSH