Sustainable Synthesis of Pure Silica Zeolites from a Combined Strategy of Zeolite Seeding and Alcohol Filling.
seeding
silica
sustainable synthesis
zeolites
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
26 Aug 2019
26 Aug 2019
Historique:
received:
26
05
2019
pubmed:
10
7
2019
medline:
10
7
2019
entrez:
9
7
2019
Statut:
ppublish
Résumé
Currently, the synthesis of pure silica zeolites always requires the presence of organic structure-directing agents (OSDAs), which direct the assembly pathway and ultimately fill the pore space. A sustainable route is now reported for synthesizing pure silica zeolites in the absence of OSDAs from a combined strategy of zeolite seeding and alcohol filling, where the zeolite seeds direct crystallization of zeolite crystals from amorphous silica, while the alcohol is served as pore filling in the zeolites. Very importantly, the alcohol could be fully washed out from zeolite pores by water at room temperature, which completely avoids calcination at high temperature for removal of OSDAs in the synthesis of pure silica zeolites.
Identifiants
pubmed: 31283076
doi: 10.1002/anie.201906559
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
12138-12142Subventions
Organisme : National Key Research and Development Program of China
ID : 2017YFB0702803
Organisme : National Natural Science Foundation of China
ID : 21703203, 21802053, 21673282 and 21673205
Informations de copyright
© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.
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