Analogue spectra for impact ionization mass spectra of water ice grains obtained at different impact speeds in space.
Journal
Rapid communications in mass spectrometry : RCM
ISSN: 1097-0231
Titre abrégé: Rapid Commun Mass Spectrom
Pays: England
ID NLM: 8802365
Informations de publication
Date de publication:
30 Nov 2019
30 Nov 2019
Historique:
received:
22
02
2019
revised:
12
06
2019
accepted:
30
06
2019
pubmed:
10
7
2019
medline:
10
7
2019
entrez:
10
7
2019
Statut:
ppublish
Résumé
Detecting ice grains with impact ionization mass spectrometers in space provides information about the compositions of ice grains and their sources. Depending on the impact speeds of the ice grains onto the metal target of a mass spectrometer, ionization conditions can vary substantially, resulting in changes to the appearance of the resulting mass spectra. Here we accurately reproduce mass spectra of water ice grains, recorded with the Cosmic Dust Analyzer (CDA) on board the Cassini spacecraft at typical impact speeds ranging between 4 km/s to 21 km/s, with a laboratory analogue experiment. In this Laser-Induced Liquid Beam Ion Desorption (LILBID) approach, a μm-sized liquid water beam is irradiated with a pulsed infrared laser, desorbing charged analyte and solvent aggregates and isolated ions, which are subsequently analyzed in a time-of-flight (TOF) mass spectrometer. We show that our analogue experiment can reproduce impact ionization mass spectra of ice grains obtained over a wide range of impact speeds, aiding the quantitative analyses of mass spectra from space. Spectra libraries created with the LILBID experiment will be a vital tool for inferring the composition of ice grains from mass spectra recorded by both past and future impact ionization mass spectrometers (e.g. the SUrface Dust Analyzer (SUDA) onboard NASA's Europa Clipper Mission or detectors on a future Enceladus Mission).
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
1751-1760Subventions
Organisme : Deutsche Forschungsgemeinschaft
ID : AB 63/9-1
Organisme : Deutsche Forschungsgemeinschaft
ID : PO 1015/2-1
Organisme : Deutsche Forschungsgemeinschaft
ID : PO 1015/3-1
Organisme : Deutsche Forschungsgemeinschaft
ID : PO 1015/4-1
Organisme : H2020 European Research Council
ID : 724908-Habitat OASIS
Informations de copyright
© 2019 John Wiley & Sons, Ltd.
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