Development and validation of a physiologically based kinetic model for starting up and operation of the biological gas desulfurization process under haloalkaline conditions.

Biological gas desulfurization Flavocytochrome c Physiologically based kinetics Sulfide-quinone oxidoreductase Sulfur-oxidizing bacteria

Journal

Water research X
ISSN: 2589-9147
Titre abrégé: Water Res X
Pays: England
ID NLM: 101742109

Informations de publication

Date de publication:
01 Aug 2019
Historique:
received: 04 04 2019
revised: 28 06 2019
accepted: 01 07 2019
entrez: 24 7 2019
pubmed: 25 7 2019
medline: 25 7 2019
Statut: epublish

Résumé

Hydrogen sulfide is a toxic and corrosive gas that must be removed from gaseous hydrocarbon streams prior to combustion. This paper describes a gas biodesulfurization process where sulfur-oxidizing bacteria (SOB) facilitate sulfide conversion to both sulfur and sulfate. In order to optimize the formation of sulfur, it is crucial to understand the relations between the SOB microbial composition, kinetics of biological and abiotic sulfide oxidation and the effects on the biodesulfurization process efficiency. Hence, a physiologically based kinetic model was developed for four different inocula. The resulting model can be used as a tool to evaluate biodesulfurization process performance. The model relies on a ratio of two key enzymes involved in the sulfide oxidation process, i.e., flavocytochrome

Identifiants

pubmed: 31334497
doi: 10.1016/j.wroa.2019.100035
pii: S2589-9147(19)30071-4
pii: 100035
pmc: PMC6614595
doi:

Types de publication

Journal Article

Langues

eng

Pagination

100035

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Auteurs

Karine Kiragosyan (K)

Wetsus, European Centre of Excellence for Sustainable Water Technology, Oostergoweg 9, 8911, MA, Leeuwarden, the Netherlands.
Environmental Technology, Wageningen University, P.O. Box 17, 6700, AA, Wageningen, the Netherlands.

Johannes B M Klok (JBM)

Wetsus, European Centre of Excellence for Sustainable Water Technology, Oostergoweg 9, 8911, MA, Leeuwarden, the Netherlands.
Environmental Technology, Wageningen University, P.O. Box 17, 6700, AA, Wageningen, the Netherlands.
Paqell B.V., Reactorweg 301, 3542, AD, Utrecht, the Netherlands.

Karel J Keesman (KJ)

Wetsus, European Centre of Excellence for Sustainable Water Technology, Oostergoweg 9, 8911, MA, Leeuwarden, the Netherlands.
Biobased Chemistry & Technology, Wageningen University, P.O. Box 17, 6700, AA, Wageningen, the Netherlands.

Pawel Roman (P)

Wetsus, European Centre of Excellence for Sustainable Water Technology, Oostergoweg 9, 8911, MA, Leeuwarden, the Netherlands.

Albert J H Janssen (AJH)

Environmental Technology, Wageningen University, P.O. Box 17, 6700, AA, Wageningen, the Netherlands.
Shell, Oostduinlaan 2, 2596, M the Hague, the Netherlands.

Classifications MeSH