Hierarchical Coherent Phonons in a Superatomic Semiconductor.

2D materials coherent phonons hierarchical structures superatomic semiconductors ultrafast spectroscopy

Journal

Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358

Informations de publication

Date de publication:
Sep 2019
Historique:
received: 20 05 2019
revised: 25 06 2019
pubmed: 26 7 2019
medline: 26 7 2019
entrez: 26 7 2019
Statut: ppublish

Résumé

The coupling of phonons to electrons and other phonons plays a defining role in material properties, such as charge and energy transport, light emission, and superconductivity. In atomic solids, phonons are delocalized over the 3D lattice, in contrast to molecular solids where localized vibrations dominate. Here, a hierarchical semiconductor that expands the phonon space by combining localized 0D modes with delocalized 2D and 3D modes is described. This material consists of superatomic building blocks (Re

Identifiants

pubmed: 31342595
doi: 10.1002/adma.201903209
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e1903209

Subventions

Organisme : Air Force Office of Scientific Research
ID : FA9550-18-1-0020
Organisme : National Science Foundation
ID : DMR-1420634
Organisme : National Science Foundation
ID : DMR-1751949
Organisme : National Science Foundation
ID : ACI-1548562
Organisme : National Science Foundation
ID : DGE 11-44155
Organisme : U.S. Department of Defense
Organisme : Feodor Lynen Fellowship
Organisme : NSF
ID : DMR-1420634
Organisme : NSF
ID : DMR-1751949
Organisme : NSF
ID : ACI-1548562
Organisme : NSF
ID : DGE 11-44155

Informations de copyright

© 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

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Auteurs

Kihong Lee (K)

Department of Chemistry, Columbia University, New York, NY, 10027, USA.

Sebastian F Maehrlein (SF)

Department of Chemistry, Columbia University, New York, NY, 10027, USA.

Xinjue Zhong (X)

Department of Chemistry, Columbia University, New York, NY, 10027, USA.

Daniele Meggiolaro (D)

Computational Laboratory for Hybrid/Organic Photovoltaics (CLHYO), CNR-ISTM, Via Elce di Sotto 8, I-06123, Perugia, Italy.
D3-CompuNet, Istituto Italiano di Tecnologia, Via Morego 30, 16163, Genova, Italy.

Jake C Russell (JC)

Department of Chemistry, Columbia University, New York, NY, 10027, USA.

Douglas A Reed (DA)

Department of Chemistry, Columbia University, New York, NY, 10027, USA.

Bonnie Choi (B)

Department of Chemistry, Columbia University, New York, NY, 10027, USA.

Filippo De Angelis (F)

Computational Laboratory for Hybrid/Organic Photovoltaics (CLHYO), CNR-ISTM, Via Elce di Sotto 8, I-06123, Perugia, Italy.
D3-CompuNet, Istituto Italiano di Tecnologia, Via Morego 30, 16163, Genova, Italy.

Xavier Roy (X)

Department of Chemistry, Columbia University, New York, NY, 10027, USA.

Xiaoyang Zhu (X)

Department of Chemistry, Columbia University, New York, NY, 10027, USA.

Classifications MeSH