Natural Born Laser Dyes: Excited-State Intramolecular Proton Transfer (ESIPT) Emitters and Their Use in Random Lasing Studies.

ESIPT ab initio calculations excited states fluorescence random lasing

Journal

Nanomaterials (Basel, Switzerland)
ISSN: 2079-4991
Titre abrégé: Nanomaterials (Basel)
Pays: Switzerland
ID NLM: 101610216

Informations de publication

Date de publication:
30 Jul 2019
Historique:
received: 27 06 2019
revised: 21 07 2019
accepted: 25 07 2019
entrez: 2 8 2019
pubmed: 2 8 2019
medline: 2 8 2019
Statut: epublish

Résumé

A series of five excited-state intramolecular proton transfer (ESIPT) emitters based on a 2-(2'-hydroxyphenyl) benzoxazole (HBO) scaffold, functionalized with a mono-or bis-(trialkylsilyl) acetylene extended spacer are presented. Investigation of their photophysical properties in solution and in the solid-state in different matrix, along with ab initio calculations gave useful insights into their optical behavior. Random lasing studies were conducted on a series of PMMA doped thin films, showing the presence of stimulated emission above the threshold of pumping energy density (ρth ≈ 0.5-2.6 mJ cm

Identifiants

pubmed: 31366091
pii: nano9081093
doi: 10.3390/nano9081093
pmc: PMC6723810
pii:
doi:

Types de publication

Journal Article

Langues

eng

Subventions

Organisme : Narodowe Centrum Nauki
ID : 2016/21/B/ST8/00468

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Auteurs

Julien Massue (J)

Institut de Chimie et Procédés pour l'Energie, l'Environnement et la Santé (ICPEES), UMR CNRS 7515, Ecole Européenne de Chimie, Polymères et Matériaux (ECPM), 25 Rue Becquerel, CEDEX 02, 67087 Strasbourg, France. massue@unistra.fr.

Thibault Pariat (T)

Institut de Chimie et Procédés pour l'Energie, l'Environnement et la Santé (ICPEES), UMR CNRS 7515, Ecole Européenne de Chimie, Polymères et Matériaux (ECPM), 25 Rue Becquerel, CEDEX 02, 67087 Strasbourg, France.

Pauline M Vérité (P)

CEISAM, UMR CNRS 6230, BP 92208, 2 rue de la Houssinière, CEDEX 03, 44322 Nantes, France.

Denis Jacquemin (D)

CEISAM, UMR CNRS 6230, BP 92208, 2 rue de la Houssinière, CEDEX 03, 44322 Nantes, France. Denis.Jacquemin@univ-nantes.fr.

Martyna Durko (M)

Advanced Materials Engineering and Modeling Group, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, 50-370 Wroclaw, Poland.

Tarek Chtouki (T)

Advanced Materials Engineering and Modeling Group, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, 50-370 Wroclaw, Poland.

Lech Sznitko (L)

Advanced Materials Engineering and Modeling Group, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, 50-370 Wroclaw, Poland.

Jaroslaw Mysliwiec (J)

Advanced Materials Engineering and Modeling Group, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, 50-370 Wroclaw, Poland. jaroslaw.mysliwiec@pwr.edu.pl.

Gilles Ulrich (G)

Institut de Chimie et Procédés pour l'Energie, l'Environnement et la Santé (ICPEES), UMR CNRS 7515, Ecole Européenne de Chimie, Polymères et Matériaux (ECPM), 25 Rue Becquerel, CEDEX 02, 67087 Strasbourg, France.

Classifications MeSH