Tuning the Chemistry of Organonitrogen Compounds for Promoting All-Organic Anionic Rechargeable Batteries.
batteries
organic batteries
redox chemistry
zwitterions
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
28 Oct 2019
28 Oct 2019
Historique:
received:
08
07
2019
revised:
08
08
2019
pubmed:
21
8
2019
medline:
21
8
2019
entrez:
21
8
2019
Statut:
ppublish
Résumé
The ever-increasing demand for rechargeable batteries induces significant pressure on the worldwide metal supply, depleting resources and increasing costs and environmental concerns. In this context, developing the chemistry of anion-inserting electrode organic materials could promote the fabrication of molecular (metal-free) rechargeable batteries. However, few examples have been reported because little effort has been made to develop such anionic-ion batteries. Here we show the design of two anionic host electrode materials based on the N-substituted salts of azaaromatics (zwitterions). A combination of NMR, EDS, FTIR spectroscopies coupled with thermal analyses and single-crystal XRD allowed a thorough structural and chemical characterization of the compounds. Thanks to a reversible electrochemical activity located at an average potential of 2.2 V vs. Li
Identifiants
pubmed: 31429162
doi: 10.1002/anie.201908475
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
15680-15684Informations de copyright
© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.
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