A new method for quantifying causative and diagnostic markers of methylenecyclopropylglycine poisoning.

AM, atypical myopathy Ackee fruit Acquired multiple acyl-CoA dehydrogenase deficiency HGA, hypoglycin A Hypoglycin A (PubChem CID: 9081) Litchi MCPA-G, methylenecyclopropylacetyl glycine MCPF, methylenecyclopropylformate MCPF-G, methylenecyclopropylformyl glycine MCPG, methylenecyclopropylglycine Methylenecyclopropylacetyl glycine (PubChem: 6429414) Methylenecyclopropylformate Methylenecyclopropylformyl glycine (PubChem: 129713646) Methylenecyclopropylglycine Methylenecyclopropylglycine (PubChem CID: 142776) Sapindaceae

Journal

Toxicology reports
ISSN: 2214-7500
Titre abrégé: Toxicol Rep
Pays: Ireland
ID NLM: 101630272

Informations de publication

Date de publication:
2019
Historique:
received: 28 03 2019
revised: 29 07 2019
accepted: 02 08 2019
entrez: 24 8 2019
pubmed: 24 8 2019
medline: 24 8 2019
Statut: epublish

Résumé

Up to now quantification of hypoglycin A in serum and urine in the range of nmols to μmols per liter plus the measurement of accumulated acyl conjugates have been used for the diagnosis of poisoning by fruits or seeds of Methylenecyclopropylglycine was extracted from serum and urine of a volunteer by a methanolic solution containing labeled methylenecyclopropylglycine as internal standard. UPLC-MS/MS analysis was performed after butylation. Lower limits of detection and quantification were found at 0.5 and 2.5 nmol/L respectively in both urine and serum for each of two isomers, linearity of results (r Quantification of methylenecyclopropylglycine can be successfully integrated into our established analytical procedure used for clinical diagnosis of

Sections du résumé

BACKGROUND BACKGROUND
Up to now quantification of hypoglycin A in serum and urine in the range of nmols to μmols per liter plus the measurement of accumulated acyl conjugates have been used for the diagnosis of poisoning by fruits or seeds of
METHOD METHODS
Methylenecyclopropylglycine was extracted from serum and urine of a volunteer by a methanolic solution containing labeled methylenecyclopropylglycine as internal standard. UPLC-MS/MS analysis was performed after butylation.
RESULTS RESULTS
Lower limits of detection and quantification were found at 0.5 and 2.5 nmol/L respectively in both urine and serum for each of two isomers, linearity of results (r
CONCLUSIONS CONCLUSIONS
Quantification of methylenecyclopropylglycine can be successfully integrated into our established analytical procedure used for clinical diagnosis of

Identifiants

pubmed: 31440457
doi: 10.1016/j.toxrep.2019.08.002
pii: S2214-7500(19)30185-4
pmc: PMC6699453
doi:

Types de publication

Journal Article

Langues

eng

Pagination

803-808

Déclaration de conflit d'intérêts

None.

Références

Biochemistry. 2002 Feb 12;41(6):1843-52
pubmed: 11827529
Biochim Biophys Acta. 1976 Jan 23;422(1):8-14
pubmed: 1247597
Biochem J. 1962 Mar;82:385-9
pubmed: 13901296
Biochim Biophys Acta. 2006 Dec;1763(12):1413-26
pubmed: 17028011
Neuromuscul Disord. 2008 May;18(5):355-64
pubmed: 18406615
Org Lett. 2008 Aug 7;10(15):3355-8
pubmed: 18611036
J Chromatogr B Analyt Technol Biomed Life Sci. 2009 Aug 1;877(23):2198-207
pubmed: 19179125
Biochem J. 1991 Mar 1;274 ( Pt 2):395-400
pubmed: 2006907
J Vet Intern Med. 2012 Jul-Aug;26(4):1012-8
pubmed: 22708588
Emerg Infect Dis. 2012 Nov;18(11):1817-24
pubmed: 23092599
Equine Vet J. 2013 Jul;45(4):419-26
pubmed: 23167695
Equine Vet J. 2014 Mar;46(2):146-9
pubmed: 23773055
MMWR Morb Mortal Wkly Rep. 2015 Jan 30;64(3):49-53
pubmed: 25632950
Science. 2015 Apr 3;348(6230):15-6
pubmed: 25838358
Chem Res Toxicol. 2015 Sep 21;28(9):1753-9
pubmed: 26328472
J Vet Diagn Invest. 2016 Mar;28(2):98-104
pubmed: 26965229
J Agric Food Chem. 2016 Jul 13;64(27):5607-13
pubmed: 27367968
J Chromatogr B Analyt Technol Biomed Life Sci. 2016 Sep 1;1029-1030:169-173
pubmed: 27433981
Lancet Glob Health. 2017 Apr;5(4):e458-e466
pubmed: 28153514
J Agric Food Chem. 2017 Mar 29;65(12):2603-2608
pubmed: 28290200
Toxicol Rep. 2017 Mar 29;4:181-187
pubmed: 28959639
Emerg Infect Dis. 2018 Aug;24(8):1435-1443
pubmed: 30014832
Experientia. 1985 Dec 15;41(12):1622-3
pubmed: 3935481
Proc Natl Acad Sci U S A. 1971 Jan;68(1):20-4
pubmed: 5276292

Auteurs

Johannes Sander (J)

Screening-Labor Hannover, Ronnenberg, Germany.

Michael Terhardt (M)

Screening-Labor Hannover, Ronnenberg, Germany.

Stefanie Sander (S)

Screening-Labor Hannover, Ronnenberg, Germany.

Sabine Aboling (S)

Institute for Animal Nutrition, University of Veterinary Medicine Hannover, Foundation, Hannover, Germany.

Nils Janzen (N)

Screening-Labor Hannover, Ronnenberg, Germany.
Department of Clinical Chemistry, Hannover Medical School, Hannover, Germany.

Classifications MeSH