Uranium sequestration in sediment at an iron-rich contaminated site at Oak Ridge, Tennessee via. bioreduction followed by reoxidation.


Journal

Journal of environmental sciences (China)
ISSN: 1001-0742
Titre abrégé: J Environ Sci (China)
Pays: Netherlands
ID NLM: 100967627

Informations de publication

Date de publication:
Nov 2019
Historique:
received: 07 04 2019
revised: 29 05 2019
accepted: 30 05 2019
entrez: 1 9 2019
pubmed: 1 9 2019
medline: 11 9 2019
Statut: ppublish

Résumé

This study evaluated uranium sequestration performance in iron-rich (30 g/kg) sediment via bioreduction followed by reoxidation. Field tests (1383 days) at Oak Ridge, Tennessee demonstrated that uranium contents in sediments increased after bioreduced sediments were re-exposed to nitrate and oxygen in contaminated groundwater. Bioreduction of contaminated sediments (1200 mg/kg U) with ethanol in microcosm reduced aqueous U from 0.37 to 0.023 mg/L. Aliquots of the bioreduced sediment were reoxidized with O

Identifiants

pubmed: 31471022
pii: S1001-0742(19)31063-0
doi: 10.1016/j.jes.2019.05.028
pii:
doi:

Substances chimiques

Soil Pollutants, Radioactive 0
Uranium 4OC371KSTK

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

156-167

Informations de copyright

Copyright © 2019. Published by Elsevier B.V.

Auteurs

Peng-Song Li (PS)

Department of Civil and Environmental Engineering, William & Cloy Codiga Resource Recovery Center, Center for Sustainable Development & Global Competitiveness, Stanford University, Stanford, CA 94305-4020, USA; Key Laboratory for Heavy Metal Pollution Control and Reutilization, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen 518055, China; Institute of New Energy Technology, Tsinghua University, Beijing 100084, China.

Wei-Min Wu (WM)

Department of Civil and Environmental Engineering, William & Cloy Codiga Resource Recovery Center, Center for Sustainable Development & Global Competitiveness, Stanford University, Stanford, CA 94305-4020, USA. Electronic address: wei-min.wu@stanford.edu.

Debra H Phillips (DH)

School of Natural and Built Environment, Queen's University Belfast, Belfast BT9 5AG, Northern Ireland, UK.

David B Watson (DB)

Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, P.O. Box 2008, TN 37831, USA.

Shelly Kelly (S)

EXAFS Analysis, Bolingbrook, IL 60440, USA.

Bing Li (B)

Department of Civil and Environmental Engineering, William & Cloy Codiga Resource Recovery Center, Center for Sustainable Development & Global Competitiveness, Stanford University, Stanford, CA 94305-4020, USA; Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, P.O. Box 2008, TN 37831, USA; Department of Civil Engineering, The University of Hong Kong, Hong Kong, China.

Tonia Mehlhorn (T)

Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, P.O. Box 2008, TN 37831, USA.

Kenneth Lowe (K)

Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, P.O. Box 2008, TN 37831, USA.

Jennifer Earles (J)

Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, P.O. Box 2008, TN 37831, USA.

Hu-Chun Tao (HC)

Key Laboratory for Heavy Metal Pollution Control and Reutilization, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen 518055, China.

Tong Zhang (T)

Department of Civil Engineering, The University of Hong Kong, Hong Kong, China.

Craig S Criddle (CS)

Department of Civil and Environmental Engineering, William & Cloy Codiga Resource Recovery Center, Center for Sustainable Development & Global Competitiveness, Stanford University, Stanford, CA 94305-4020, USA. Electronic address: ccriddle@stanford.edu.

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Classifications MeSH