Interpretation and Automatic Generation of Fermi-Orbital Descriptors.

FLO-SIC Linnett double-quartet theory chemical bonding density functional theory

Journal

Journal of computational chemistry
ISSN: 1096-987X
Titre abrégé: J Comput Chem
Pays: United States
ID NLM: 9878362

Informations de publication

Date de publication:
15 Dec 2019
Historique:
received: 19 02 2019
revised: 13 08 2019
accepted: 14 08 2019
pubmed: 11 9 2019
medline: 11 9 2019
entrez: 11 9 2019
Statut: ppublish

Résumé

We present an interpretation of Fermi-orbital descriptors (FODs) and argue that these descriptors carry chemical bonding information. We show that a bond order derived from these FODs agrees well with reference values, and highlight that optimized FOD positions used within the Fermi-Löwdin orbital self-interaction correction (FLO-SIC) method correspond to expectations from Linnett's double-quartet theory, which is an extension of Lewis theory. This observation is independent of the underlying exchange-correlation functional, which is shown using the local spin density approximation, the Perdew-Burke-Ernzerhof generalized gradient approximation (GGA), and the strongly constrained and appropriately normed meta-GGA. To make FOD positions generally accessible, we propose and discuss four independent methods for the generation of Fermi-orbital descriptors, their implementation as well as their advantages and drawbacks. In particular, we introduce a re-implementation of the electron force field, an approach based on the centers of mass of orbital densities, a Monte Carlo-based algorithm, and a method based on Lewis-like bonding information. All results are summarized with respect to future developments of FLO-SIC and related methods. © 2019 The Authors. Journal of Computational Chemistry published by Wiley Periodicals, Inc.

Identifiants

pubmed: 31503364
doi: 10.1002/jcc.26062
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

2843-2857

Subventions

Organisme : U. S. Department of Energy
Organisme : Office of Science
Organisme : Office of Basic Energy Sciences
ID : #DE-SC0018331
Organisme : Deutsche Forschungsgemeinschaft
ID : KO 1924/9-1

Informations de copyright

© 2019 The Authors. Journal of Computational Chemistry published by Wiley Periodicals, Inc.

Références

P. Hohenberg, W. Kohn, Phys. Rev. 1964, 136, B864.
W. Kohn, L. J. Sham, Phys. Rev. 1965, 140, A1133.
J. Kortus, M. R. Pederson, T. Baruah, N. Bernstein, C. Hellberg, Polyhedron 2003, 22, 1871.
C. Loose, E. Ruiz, J. Cirera, J. Cano, S. Alvarez, and J. Kortus, in APS Meeting Abstracts, Royal Society of Chemistry, 2008.
J. Cirera, E. Ruiz, S. Alvarez, F. Neese, J. Kortus, Chem. A Eur. J. 2009, 15, 4078.
K. Rühlig, A. Abylaikhan, A. Aliabadi, V. Kataev, S. Liebing, S. Schwalbe, K. Trepte, C. Ludt, J. Kortus, B. Büchner, T. Rüffer, H. Lang, Dalton Trans. 2017, 46, 3963.
S. Liebing, C. Martin, K. Trepte, J. Kortus, Phys. Rev. B 2015, 91, 155421.
J. Kortus, I. I. Mazin, K. D. Belashchenko, V. P. Antropov, L. L. Boyer, Phys. Rev. Lett. 2001, 86, 4656.
A. Y. Liu, I. I. Mazin, J. Kortus, Phys. Rev. Lett. 2001, 87, 087005.
J. Kortus, O. V. Dolgov, R. K. Kremer, A. A. Golubov, Phys. Rev. Lett. 2005, 94, 027002.
K. Trepte, S. Schwalbe, G. Seifert, Phys. Chem. Chem. Phys. 2015, 17, 17122.
S. Schwalbe, K. Trepte, G. Seifert, J. Kortus, Phys. Chem. Chem. Phys. 2016, 18, 8075.
K. Trepte, J. Schaber, S. Schwalbe, F. Drache, I. Senkovska, S. Kaskel, J. Kortus, E. Brunner, G. Seifert, Phys. Chem. Chem. Phys. 2017, 19, 10020.
K. Trepte, S. Schwalbe, J. Schaber, S. Krause, I. Senkovska, S. Kaskel, E. Brunner, J. Kortus, G. Seifert, Phys. Chem. Chem. Phys. 2018, 20, 25039.
S. Schwalbe, R. Wirnata, R. Starke, G. A. Schober, J. Kortus, Phys. Rev. B 2016, 94, 205130.
A. Ruzsinszky, J. P. Perdew, G. I. Csonka, J. Phys. Chem. A 2005, 109, 11006.
J. P. Perdew, Int. J. Quantum Chem. 1985, 28, 497.
V. Maslen, Proc. Phys. Soc. Section A 1956, 69, 734.
M. Buijse, E. Baerends, Mol. Phys. 2002, 100, 401.
A. Becke, M. Roussel, Phys. Rev. A 1989, 39, 3761.
H. Bahmann, Phd thesis: Implementation, Development and Assessment of Local Hybrid Density Functionals. 2011.
A. D. Becke, J. Chem. Phys. 2013, 138, 074109.
J. Přecechtělová, H. Bahmann, M. Kaupp, M. Ernzerhof, J. Chem. Phys. 2014, 141, 111102.
H. Bahmann, Y. Zhou, M. Ernzerhof, J. Chem. Phys. 2016, 145, 124104.
R. F. W. Bader, A. Streitwieser, A. Neuhaus, K. E. Laidig, P. Speers, J. Am. Chem. Soc. 1996, 118, 4959.
D. R. Hartree, Math. Proc. Camb. Philos. Soc. 1928, 24, 89.
V. Fock, Z. Phys. 1930, 61, 126.
W. L. Luken, J. C. Culberson, Int. J. Quantum Chem. 1982, 22, 265.
W. L. Luken, D. N. Beratan, Theor. Chim. Acta 1982, 61, 265.
W. L. Luken, Croat. Chem. Acta 1984, 57, 1283.
J. P. Perdew, A. Zunger, Phys. Rev. B 1981, 23, 5048.
C. Shahi, P. Bhattarai, K. Wagle, B. Santra, S. Schwalbe, T. Hahn, J. Kortus, K. A. Jackson, J. E. Peralta, K. Trepte, S. Lehtola, N. K. Nepal, H. Myneni, B. Neupane, S. Adhikari, A. Ruzsinszky, Y. Yamamoto, T. Baruah, R. R. Zope, J. P. Perdew, J. Chem. Phys. 2019, 150, 174102.
S. Klüpfel, P. Klüpfel, H. Jónsson, Phys. Rev. A 2011, 84, 050501.
O. A. Vydrov, G. E. Scuseria, J. Chem. Phys. 2005, 122, 184107.
G. Borghi, A. Ferretti, N. L. Nguyen, I. Dabo, N. Marzari, Phys. Rev. B 2014, 90, 075135.
S. Schwalbe, T. Hahn, S. Liebing, K. Trepte, J. Kortus, J. Comput. Chem. 2018, 39, 2463.
C. D. Pemmaraju, S. Sanvito, K. Burke, Phys. Rev. B 2008, 77, 121204.
A. Ruzsinszky, J. P. Perdew, G. I. Csonka, G. E. Scuseria, O. A. Vydrov, Phys. Rev. A 2008, 77, 060502.
J. G. Harrison, R. A. Heaton, C. C. Lin, J. Phys. B 1983, 16, 2079.
M. R. Pederson, R. A. Heaton, C. C. Lin, J. Chem. Phys. 1984, 80, 1972.
E. Baerends, Phys. Rev. Lett. 2001, 87, 133004.
M. R. Pederson, A. Ruzsinszky, J. P. Perdew, J. Chem. Phys. 2014, 140, 121103.
M. R. Pederson, J. Chem. Phys. 2015, 142, 064112.
M. R. Pederson, T. Baruah, In Advances In Atomic, Molecular, and Optical Physics, Vol. 64; E. Arimondo, C. C. Lin, S. F. Yelin, Eds., Elsevier, 2015, p. 153.
Z.-h. Yang, M. R. Pederson, J. P. Perdew, Phys. Rev. A 2017, 95, 052505.
K. Trepte, S. Schwalbe, T. Hahn, J. Kortus, D.-Y. Kao, Y. Yamamoto, T. Baruah, R. R. Zope, K. P. K. Withanage, J. E. Peralta, K. A. Jackson, J. Comput. Chem. 2019, 40, 820.
W. L. Luken, J. C. Culberson, Theor. Chem. Acc. 1984, 66, 279.
P.-O. Löwdin, J. Chem. Phys. 1950, 18, 365.
J. Foster, S. Boys, Rev. Mod. Phys. 1960, 32, 300.
C. Edmiston, K. Ruedenberg, Rev. Mod. Phys. 1963, 35, 457.
J. Pipek, P. G. Mezey, J. Chem. Phys. 1989, 90, 4916.
J. P. Perdew, Y. Wang, Phys. Rev. B 1992, 45, 13244.
J. P. Perdew, K. Burke, M. Ernzerhof, Phys. Rev. Lett. 1996, 77, 3865.
J. Sun, A. Ruzsinszky, J. P. Perdew, Phys. Rev. Lett. 2015, 115, 036402.
G. N. Lewis, J. Am. Chem. Soc. 1916, 38, 762.
J. Linnett, Nature 1960, 187, 859.
J. Linnett, J. Am. Chem. Soc. 1961, 83, 2643.
J. W. Linnett, Electronic Structure of Molecules, Methuen & Co. Ltd., London, 1964.
W. B. Jensen, Educación Química 2017, 28, 74.
R. M. Martin, Electronic Structure: Basic Theory and Practical Methods, Cambridge University Press, 2004.
A. C. Cancio, M. Y. Chou, R. Q. Hood, Phys. Rev. B 2001, 64, 115112.
K. J. Giesbertz, R. van Leeuwen, U. von Barth, Phys. Rev. A 2013, 87, 022514.
P. Atkins, T. Overton, Shriver and Atkins' Inorganic Chemistry, Oxford University Press, USA, 2010.
J. Kraus, Bachelor Thesis: FLOSIC-DFT Analysis of Chemical Bonding: Application to Diatomic Molecules, 2017. DOI: https://doi.org/10.13140/RG.2.2.15045.91362.
E. D. Glendening, C. R. Landis, F. Weinhold, Wiley Interdiscip. Rev. Comput. Mol. Sci. 2012, 2, 1.
R. Gillespie, J. Chem. Educ. 1963, 40, 295.
T. A. Manz, RSC Adv. 2017, 7, 45552.
R. D. Johnson, NIST Computational Chemistry Comparison and Benchmark Database (NIST Standard Reference Database Number 101, Oct 18, 2016). http://cccbdb.nist.gov/.
A. Gindulyte, B. A. Shoemaker, B. Yu, J. He, J. Zhang, J. Chen, L. Zaslavsky, P. A. Thiessen, Q. Li, S. He, et al., Nucleic Acids Res. 2018, 47, D1102.
H. E. Pence, A. Williams, J. Chem. Educ. 2010, 87, 1123.
W. F. Luder, J. Chem. Educ. 1964, 43, 55.
S. Kale, J. Herzfeld, S. Dai, M. Blank, J. Biol. Phys. 2012, 38, 49.
S. Kale, J. Herzfeld, J. Chem. Phys. 2012, 136, 084109.
S. Ekesan, S. Kale, J. Herzfeld, J. Comput. Chem. 2014, 35, 1159.
J. T. Su, W. A. Goddard, Phys. Rev. Lett. 2007, 99, 185003.
J. T. Su, W. A. Goddard, Proc. Natl. Acad. Sci. 2009, 106, 1001.
J. T. Su, An Electron Force Field for Simulating Large Scale Excited Electron Dynamics. Dissertation (Ph.D.), California Institute of Technology, 2007. http://resolver.caltech.edu/CaltechETD:etd-05032007-151410.
A. Jaramillo-Botero, J. T. Su, A. Qi, W. A. Goddard, J. Comput. Chem. 2011, 32, 497.
A. A. Frost, R. A. Rouse, J. Am. Chem. Soc. 1968, 90, 1965.
S. Plimpton, J. Comput. Phys. 1995, 117, 1.
J. Kortus, M. R. Pederson, Phys. Rev. B 2000, 62, 5755.
M. R. Pederson, K. A. Jackson, W. E. Pickett, Phys. Rev. B 1991, 44, 3891.
M. R. Pederson, D. V. Porezag, J. Kortus, D. C. Patton, Phys. Status Solidi B 2000, 217, 197.
M. R. Pederson, K. A. Jackson, Phys. Rev. B 1991, 43, 7312.
D. V. Porezag, M. R. Pederson, Phys. Rev. A Atomic Mol. Optical Phys. 1999, 60, 2840.
J. P. Perdew, J. A. Chevary, S. H. Vosko, K. A. Jackson, M. R. Pederson, D. J. Singh, C. Fiolhais, Phys. Rev. B 1992, 46, 6671.
D. Porezag, Ph.D. Thesis, TU Chemnitz, Fakultät für Naturwissenschaften. 1997. http://archiv.tu-chemnitz.de/pub/1997/0025.
S. Schwalbe, L. Fiedler, T. Hahn, K. Trepte, J. Kraus, and J. Kortus, arXiv e-prints arXiv:1905.02631. 2019. 1905.02631.
S. Lehtola, H. Jónsson, J. Chem. Theory Comput. 2013, 9, 5365.
Q. Sun, T. C. Berkelbach, N. S. Blunt, G. H. Booth, S. Guo, Z. Li, J. Liu, J. D. McClain, E. R. Sayfutyarova, S. Sharma, S. Wouters, G. K. L. Chan, Wiley Interdiscip. Rev. Comput. Mol. Sci. 2018, 8, e1340.
Q. Sun, arXiv preprint arXiv:1610.08423. 2016.
J. R. Morris, D. M. Deaven, K. M. Ho, Phys. Rev. B 1996, 53, R1740.
S. Lehtola, M. Head-Gordon, H. Jónsson, J. Chem. Theory Comput. 2016, 12, 3195.
T. Hahn, S. Liebing, J. Kortus, M. R. Pederson, J. Chem. Phys. 2015, 143, 224104.
D.-y. Kao, K. Withanage, T. Hahn, J. Batool, J. Kortus, K. Jackson, J. Chem. Phys. 2017, 147, 164107.
G. Landrum, Rdkit: Open-Source Cheminformatics. http://www.rdkit.org.
S. Lehtola, H. Jónsson, J. Chem. Theory Comput. 2014, 10, 5324.
S. Schwalbe, L. Fiedler, K. Trepte, T. Hahn, J. Kortus, and J. Perdew, Self-Interaction Corrected Density Functional Theory is Not Straying from the Path Towards the Exact Functional, Manuscript in Preparation. 2019.
Atomic Simulation Environment, 2018. https://wiki.fysik.dtu.dk/ase/.
E. Bitzek, P. Koskinen, F. Gähler, M. Moseler, P. Gumbsch, Phys. Rev. Lett. 2006, 97, 170201.
W. F. Luder, J. Chem. Educ. 1966, 43, 55.
W. F. Luder, J. Chem. Educ. 1967, 44, 206.
S. Schwalbe, T. Gruber, K. Trepte, F. Taubert, F. Mertens, J. Kortus, Comput. Mater. Sci. 2017, 134, 48.
F. Taubert, S. Schwalbe, J. Seidel, R. Huettl, T. Gruber, R. Janot, M. Bobnar, R. Gumeniuk, F. Mertens, J. Kortus, Int. J. Mater. Res. 2017, 108, 942.

Auteurs

Sebastian Schwalbe (S)

TU Freiberg, Institute of Theoretical Physics, Leipziger Str. 23, D-09599, Freiberg, Germany.

Kai Trepte (K)

Department of Physics, Central Michigan University, Mount Pleasant, Michigan, 48859.

Lenz Fiedler (L)

TU Freiberg, Institute of Theoretical Physics, Leipziger Str. 23, D-09599, Freiberg, Germany.
Freiberg Instruments GmbH, Delfter Str.6, D-09599, Freiberg, Germany.

Alex I Johnson (AI)

Department of Physics, Central Michigan University, Mount Pleasant, Michigan, 48859.

Jakob Kraus (J)

TU Freiberg, Institute of Theoretical Physics, Leipziger Str. 23, D-09599, Freiberg, Germany.

Torsten Hahn (T)

TU Freiberg, Institute of Theoretical Physics, Leipziger Str. 23, D-09599, Freiberg, Germany.

Juan E Peralta (JE)

Department of Physics, Central Michigan University, Mount Pleasant, Michigan, 48859.

Koblar A Jackson (KA)

Department of Physics, Central Michigan University, Mount Pleasant, Michigan, 48859.

Jens Kortus (J)

TU Freiberg, Institute of Theoretical Physics, Leipziger Str. 23, D-09599, Freiberg, Germany.

Classifications MeSH