TITAN: A Code for Modeling and Generating Electric Fields-Features and Applications to Enzymatic Reactivity.

H-abstraction reaction TITAN code external electric field intrinsic electric fields local electric fields oriented electric fields

Journal

Journal of computational chemistry
ISSN: 1096-987X
Titre abrégé: J Comput Chem
Pays: United States
ID NLM: 9878362

Informations de publication

Date de publication:
05 01 2020
Historique:
received: 22 07 2019
revised: 22 08 2019
accepted: 31 08 2019
pubmed: 1 10 2019
medline: 1 4 2021
entrez: 1 10 2019
Statut: ppublish

Résumé

We present here a versatile computational code named "elecTric fIeld generaTion And maNipulation (TITAN)," capable of generating various types of external electric fields, as well as quantifying the local (or intrinsic) electric fields present in proteins and other biological systems according to Coulomb's Law. The generated electric fields can be coupled with quantum mechanics (QM), molecular mechanics (MM), QM/MM, and molecular dynamics calculations in most available software packages. The capabilities of the TITAN code are illustrated throughout the text with the help of examples. We end by presenting an application, in which the effects of the local electric field on the hydrogen transfer reaction in cytochrome P450 OleT

Identifiants

pubmed: 31568581
doi: 10.1002/jcc.26072
doi:

Substances chimiques

Cytochrome P-450 Enzyme System 9035-51-2

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

74-82

Informations de copyright

© 2019 Wiley Periodicals, Inc.

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Auteurs

Thijs Stuyver (T)

Institute of Chemistry, The Lise Meitner-Minerva Center for Computational Quantum Chemistry, Hebrew University of Jerusalem, Givat Ram Campus, Jerusalem, 91904, Israel.
Algemene Chemie, Vrije Universiteit Brussel, Pleinlaan 2, 1050, Brussels, Belgium.

Jing Huang (J)

Institute of Chemistry, The Lise Meitner-Minerva Center for Computational Quantum Chemistry, Hebrew University of Jerusalem, Givat Ram Campus, Jerusalem, 91904, Israel.
College of Environmental and Biological Engineering, Putian University, Putian, Fujian, 351100, China.

Dibyendu Mallick (D)

Institute of Chemistry, The Lise Meitner-Minerva Center for Computational Quantum Chemistry, Hebrew University of Jerusalem, Givat Ram Campus, Jerusalem, 91904, Israel.
Department of Chemistry, Presidency University, Kolkata, 700073, India.

David Danovich (D)

Institute of Chemistry, The Lise Meitner-Minerva Center for Computational Quantum Chemistry, Hebrew University of Jerusalem, Givat Ram Campus, Jerusalem, 91904, Israel.

Sason Shaik (S)

Institute of Chemistry, The Lise Meitner-Minerva Center for Computational Quantum Chemistry, Hebrew University of Jerusalem, Givat Ram Campus, Jerusalem, 91904, Israel.

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