Synthesis of magnesium-nitrogen salts of polynitrogen anions.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
04 10 2019
Historique:
received: 14 06 2019
accepted: 16 09 2019
entrez: 6 10 2019
pubmed: 6 10 2019
medline: 6 10 2019
Statut: epublish

Résumé

The synthesis of polynitrogen compounds is of fundamental importance due to their potential as environmentally-friendly high energy density materials. Attesting to the intrinsic difficulties related to their formation, only three polynitrogen ions, bulk stabilized as salts, are known. Here, magnesium and molecular nitrogen are compressed to about 50 GPa and laser-heated, producing two chemically simple salts of polynitrogen anions, MgN

Identifiants

pubmed: 31586062
doi: 10.1038/s41467-019-12530-w
pii: 10.1038/s41467-019-12530-w
pmc: PMC6778147
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

4515

Références

Phys Rev B Condens Matter. 1996 Dec 15;54(23):16317-16320
pubmed: 9985733
Nat Mater. 2004 Aug;3(8):558-63
pubmed: 15235595
Phys Chem Chem Phys. 2017 Mar 29;19(13):9246-9252
pubmed: 28322368
Inorg Chem. 2009 Oct 19;48(20):9737-41
pubmed: 19754099
Science. 2017 Jan 27;355(6323):351
pubmed: 28126772
Science. 2016 Mar 25;351(6280):aad3000
pubmed: 27013736
Phys Rev Lett. 1996 Oct 28;77(18):3865-3868
pubmed: 10062328
J Chem Phys. 2004 Dec 8;121(22):11296-300
pubmed: 15634085
Science. 2002 Jan 18;295(5554):480-1
pubmed: 11799238
Acta Crystallogr E Crystallogr Commun. 2018 Sep 07;74(Pt 10):1392-1395
pubmed: 30319786
Angew Chem Int Ed Engl. 2001 Aug 17;40(16):2947
pubmed: 12203615
Angew Chem Int Ed Engl. 2018 Mar 1;57(10):2592-2595
pubmed: 29336110
J Phys Chem Lett. 2018 Apr 5;9(7):1600-1604
pubmed: 29533665
Angew Chem Int Ed Engl. 2017 Apr 10;56(16):4512-4514
pubmed: 28328154
Angew Chem Int Ed Engl. 2002 Aug 16;41(16):3051-4
pubmed: 12203455
Nat Commun. 2018 Jul 16;9(1):2756
pubmed: 30013071
Angew Chem Int Ed Engl. 2018 Jul 16;57(29):9048-9053
pubmed: 29774981
Nature. 2017 Sep 7;549(7670):78-81
pubmed: 28847006

Auteurs

Dominique Laniel (D)

Material Physics and Technology at Extreme Conditions, Laboratory of Crystallography, University of Bayreuth, 95440, Bayreuth, Germany. dominique.laniel@uni-bayreuth.de.

Bjoern Winkler (B)

Institut für Geowissenschaften, Abteilung Kristallographie, Johann Wolfgang Goethe-Universität Frankfurt, Altenhöferallee 1, D-60438, Frankfurt am Main, Germany.

Egor Koemets (E)

Bayerisches Geoinstitut, University of Bayreuth, 95440, Bayreuth, Germany.

Timofey Fedotenko (T)

Material Physics and Technology at Extreme Conditions, Laboratory of Crystallography, University of Bayreuth, 95440, Bayreuth, Germany.

Maxim Bykov (M)

Bayerisches Geoinstitut, University of Bayreuth, 95440, Bayreuth, Germany.

Elena Bykova (E)

Photon Science, Deutsches Elektronen-Synchrotron, Notkestrasse 85, 22607, Hamburg, Germany.

Leonid Dubrovinsky (L)

Bayerisches Geoinstitut, University of Bayreuth, 95440, Bayreuth, Germany.

Natalia Dubrovinskaia (N)

Material Physics and Technology at Extreme Conditions, Laboratory of Crystallography, University of Bayreuth, 95440, Bayreuth, Germany.

Classifications MeSH