MicroNIR/Chemometrics: A new analytical platform for fast and accurate detection of Δ9-Tetrahydrocannabinol (THC) in oral fluids.


Journal

Drug and alcohol dependence
ISSN: 1879-0046
Titre abrégé: Drug Alcohol Depend
Pays: Ireland
ID NLM: 7513587

Informations de publication

Date de publication:
01 12 2019
Historique:
received: 17 05 2019
revised: 16 07 2019
accepted: 22 07 2019
pubmed: 15 10 2019
medline: 1 7 2020
entrez: 15 10 2019
Statut: ppublish

Résumé

Δ Specimens from volunteers were collected in order to consider any sources of variability in the spectral response and spiked with increasing amount of THC in order to realize predictive models to be used in real cases. Partial Least Square-Discriminant Analysis (PLS-DA) and Partial Least Square regression (PLSr) for the simultaneously detection and quantification of THC, were applied to baseline corrected spectra pre-treated by first derivative transform. Results demonstrated that MicroNIR/Chemometric platform is statistically able to identify THC abuse in simulated oral fluid samples containing THC from 10 to 100 ng/ml, with a precision and a sensitivity of about 1.51% and 0.1% respectively. The coupling MicroNIR/Chemometrics permits to simplify THC abuse monitoring for roadside drug testing or workplace surveillance and provides the rapid interpretation of results, as once the model is assessed, it can be used to process real samples in a "click-on" device.

Sections du résumé

BACKGROUND
Δ
METHODS
Specimens from volunteers were collected in order to consider any sources of variability in the spectral response and spiked with increasing amount of THC in order to realize predictive models to be used in real cases. Partial Least Square-Discriminant Analysis (PLS-DA) and Partial Least Square regression (PLSr) for the simultaneously detection and quantification of THC, were applied to baseline corrected spectra pre-treated by first derivative transform.
RESULTS
Results demonstrated that MicroNIR/Chemometric platform is statistically able to identify THC abuse in simulated oral fluid samples containing THC from 10 to 100 ng/ml, with a precision and a sensitivity of about 1.51% and 0.1% respectively.
CONCLUSIONS
The coupling MicroNIR/Chemometrics permits to simplify THC abuse monitoring for roadside drug testing or workplace surveillance and provides the rapid interpretation of results, as once the model is assessed, it can be used to process real samples in a "click-on" device.

Identifiants

pubmed: 31610296
pii: S0376-8716(19)30355-2
doi: 10.1016/j.drugalcdep.2019.107578
pii:
doi:

Substances chimiques

Analgesics, Non-Narcotic 0
Dronabinol 7J8897W37S

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

107578

Informations de copyright

Copyright © 2019 Elsevier B.V. All rights reserved.

Auteurs

Roberta Risoluti (R)

Department of Chemistry, "Sapienza" University of Rome, p.le A.Moro 5, 00185 Rome, Italy. Electronic address: roberta.risoluti@uniroma1.it.

Giuseppina Gullifa (G)

Department of Chemistry, "Sapienza" University of Rome, p.le A.Moro 5, 00185 Rome, Italy.

Alfredo Battistini (A)

Consiglio per la ricerca in agricoltura e l'analisi dell'economia agrarian, Centro di Politiche e Bioeconomia, via Pò 14, 00198, Italy.

Stefano Materazzi (S)

Department of Chemistry, "Sapienza" University of Rome, p.le A.Moro 5, 00185 Rome, Italy.

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