Water-Soluble Polymeric Carbon Nitride Colloidal Nanoparticles for Highly Selective Quasi-Homogeneous Photocatalysis.
carbon nitride
chemoselectivity
nanoparticles
photocatalysis
quasi-homogeneous catalysis
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
02 Jan 2020
02 Jan 2020
Historique:
received:
18
10
2019
pubmed:
30
10
2019
medline:
30
10
2019
entrez:
30
10
2019
Statut:
ppublish
Résumé
Heptazine-based polymeric carbon nitrides (PCN) are promising photocatalysts for light-driven redox transformations. However, their activity is hampered by low surface area resulting in low concentration of accessible active sites. Herein, we report a bottom-up preparation of PCN nanoparticles with a narrow size distribution (ca. 10±3 nm), which are fully soluble in water showing no gelation or precipitation over several months. They allow photocatalysis to be carried out under quasi-homogeneous conditions. The superior performance of water-soluble PCN, compared to conventional solid PCN, is shown in photocatalytic H
Identifiants
pubmed: 31659848
doi: 10.1002/anie.201913331
pmc: PMC6973021
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
487-495Subventions
Organisme : Deutsche Forschungsgemeinschaft
ID : 364549901
Organisme : Deutsche Forschungsgemeinschaft
ID : BE 5102/3-1
Organisme : Deutsche Forschungsgemeinschaft
ID : TU 149/8-2
Organisme : Deutsche Forschungsgemeinschaft
ID : INST 275/257-1 FUGG
Organisme : MINECO
ID : MAT2016-78155-C2-1-R
Organisme : Gobierno del Principado de Asturias
ID : GRUPIN-ID2018-170
Organisme : CICECO-Aveiro Institute of Materials
ID : UID/CTM/50011/2019
Organisme : Ministério da Ciência, Tecnologia e Ensino Superior
ID : PTDC/QEQ-QAN/6373/2014
Organisme : University of Iceland Research Fund
Organisme : Ministerium für Wissenschaft, Forschung und Kunst Baden-Württemberg
ID : INST 40/467-1 FUGG
Organisme : Alexander von Humboldt-Stiftung
Organisme : National NMR Network (PTNMR)
ID : Infrastructure Project Nº 022161
Informations de copyright
© 2019 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA.
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