An Unexpected Transannular [4+2] Cycloaddition during the Total Synthesis of (+)-Norcembrene 5.

Diels-Alder reaction ring-closing metathesis terpenoids total synthesis transannular cycloaddition

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
27 03 2020
Historique:
received: 02 10 2019
revised: 04 11 2019
pubmed: 22 11 2019
medline: 22 11 2019
entrez: 22 11 2019
Statut: ppublish

Résumé

We report a concise and versatile total synthesis of the diterpenoid (+)-norcembrene 5 from simple building blocks. Ring-closing metathesis and an auxiliary-directed 1,4-addition are the key steps of our synthetic route. During the synthesis, an unprecedented, highly oxidized pentacyclic structural motif was established from a furanocembranoid through transannular [4+2] cycloaddition.

Identifiants

pubmed: 31750980
doi: 10.1002/anie.201912613
pmc: PMC7155007
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

5521-5525

Informations de copyright

© 2019 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA.

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Auteurs

Michael Breunig (M)

Department of Chemistry, University of Konstanz, Universitätsstrasse 10, 78464, Konstanz, Germany.

Po Yuan (P)

Department of Chemistry, University of Konstanz, Universitätsstrasse 10, 78464, Konstanz, Germany.

Tanja Gaich (T)

Department of Chemistry, University of Konstanz, Universitätsstrasse 10, 78464, Konstanz, Germany.

Classifications MeSH