Heterogeneity of dynamics in a modulated colloidal liquid.
Journal
Journal of physics. Condensed matter : an Institute of Physics journal
ISSN: 1361-648X
Titre abrégé: J Phys Condens Matter
Pays: England
ID NLM: 101165248
Informations de publication
Date de publication:
20 Mar 2020
20 Mar 2020
Historique:
pubmed:
26
11
2019
medline:
26
11
2019
entrez:
26
11
2019
Statut:
ppublish
Résumé
We study the dynamics of a system of two dimensional colloidal particles subjected to a spatially periodic external potential using Brownian dynamics simulations. We characterize the dynamics in the system by the mean square displacements and the self-van Hove function. The static density plots suggest that system gets into modulated liquid phase in presence of the external potential. We find that diffusion coefficients, obtained from long time mean sqaure displacements, decay exponentially with increasing potential strength. The self-van Hove functions computed from the distribution of particle displacemets in a given time interval show non-gaussian behaviour in directions both parallel and transverse to the external modulation. This suggests heterogeneous dynamics and is supported by particle mobilities and residence times.
Identifiants
pubmed: 31766036
doi: 10.1088/1361-648X/ab5b29
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM