Visualization Analysis of Pt and Co Species in Degraded Pt

PEFC Pt3Co/C degradation process Pt and Co chemical species maps dissolved Pt2+ and Co2+ maps same-view nano-XAFS/STEM-EDS combination technique visualization analysis

Journal

ACS applied materials & interfaces
ISSN: 1944-8252
Titre abrégé: ACS Appl Mater Interfaces
Pays: United States
ID NLM: 101504991

Informations de publication

Date de publication:
15 Jan 2020
Historique:
pubmed: 17 12 2019
medline: 17 12 2019
entrez: 17 12 2019
Statut: ppublish

Résumé

In order to obtain a suitable design policy for the development of a next-generation polymer electrolyte fuel cell, we performed a visualization analysis of Pt and Co species following aging and degradation processes in membrane-electrode assembly (MEA), using a same-view. Nano-X-ray absorption fine structure (XAFS)/Scanning transmission electron microscope (STEM)-energy dispersive X-ray spectroscopy (EDS) technique that we developed to elucidate durability factors and degradation mechanisms of a MEA Pt

Identifiants

pubmed: 31841306
doi: 10.1021/acsami.9b16393
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

2299-2312

Auteurs

Shinobu Takao (S)

Innovation Research Center for Fuel Cells , The University of Electro-Communications , Chofugaoka, Chofu , Tokyo 182-8585 , Japan.

Oki Sekizawa (O)

Innovation Research Center for Fuel Cells , The University of Electro-Communications , Chofugaoka, Chofu , Tokyo 182-8585 , Japan.
Japan Synchrotron Radiation Research Institute , Spring-8 , Sayo , Hyogo 679-5198 , Japan.

Kotaro Higashi (K)

Innovation Research Center for Fuel Cells , The University of Electro-Communications , Chofugaoka, Chofu , Tokyo 182-8585 , Japan.

Gabor Samjeské (G)

Department of Chemistry, Graduate School of Science , Nagoya University , Chikusa, Nagoya , Aichi 464-8602 , Japan.

Takuma Kaneko (T)

Innovation Research Center for Fuel Cells , The University of Electro-Communications , Chofugaoka, Chofu , Tokyo 182-8585 , Japan.

Tomohiro Sakata (T)

Innovation Research Center for Fuel Cells , The University of Electro-Communications , Chofugaoka, Chofu , Tokyo 182-8585 , Japan.

Takashi Yamamoto (T)

Department of Mathematical and Material Sciences, Faculty of Integrated Arts and Sciences , The University of Tokushima , Minamijosanjima, Tokushima 770-8502 , Japan.

Tomoya Uruga (T)

Innovation Research Center for Fuel Cells , The University of Electro-Communications , Chofugaoka, Chofu , Tokyo 182-8585 , Japan.
Japan Synchrotron Radiation Research Institute , Spring-8 , Sayo , Hyogo 679-5198 , Japan.

Yasuhiro Iwasawa (Y)

Innovation Research Center for Fuel Cells , The University of Electro-Communications , Chofugaoka, Chofu , Tokyo 182-8585 , Japan.
Department of Engineering Science, Graduate School of Informatics and Engineering , The University of Electro-Communications , Chofugaoka, Chofu , Tokyo 182-8585 , Japan.

Classifications MeSH