Towards the Molecular Design of Spin-Crossover Complexes of 2,6-Bis(pyrazol-3-yl)pyridines.

2,6-bis(pyrazol-3-yl)pyridine NMR spectroscopy iron(II) complexes molecular design spin-crossover

Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
04 May 2020
Historique:
received: 06 01 2020
pubmed: 23 1 2020
medline: 23 1 2020
entrez: 23 1 2020
Statut: ppublish

Résumé

The molecular design of spin-crossover complexes relies on controlling the spin state of a transition metal ion by proper chemical modifications of the ligands. Herein, the first N,N'-disubstituted 2,6-bis(pyrazol-3-yl)pyridines (3-bpp) are reported that, against the common wisdom, induce a spin-crossover in otherwise high-spin iron(II) complexes by increasing the steric demand of a bulky substituent, an ortho-functionalized phenyl group. As N,N'-disubstituted 3-bpp complexes have no pendant NH groups that make their spin state extremely sensitive to the environment, the proposed ligand design, which may be applicable to isomeric 1-bpp or other families of popular bi-, tri- and higher denticity ligands, opens the way for their molecular design as spin-crossover compounds for future breakthrough applications.

Identifiants

pubmed: 31967374
doi: 10.1002/chem.202000047
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

5629-5638

Subventions

Organisme : Russian Science Foundation
ID : 17-13-01456

Informations de copyright

© 2020 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

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Auteurs

Igor Nikovskiy (I)

A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilova Str., 28, 119991, Moscow, Russia.

Alexander Polezhaev (A)

A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilova Str., 28, 119991, Moscow, Russia.
Bauman Moscow State Technical University, 2nd Baumanskaya Str. 5, 105005, Moscow, Russia.

Valentin Novikov (V)

A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilova Str., 28, 119991, Moscow, Russia.
Moscow Institute of Physics and Technology, Institutskiy per., 9, Dolgoprudny, 141700, Moscow Region, Russia.

Dmitry Aleshin (D)

A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilova Str., 28, 119991, Moscow, Russia.
Mendeleev University of Chemical Technology of Russia, Miusskaya pl., 9, 125047, Moscow, Russia.

Alexander Pavlov (A)

A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilova Str., 28, 119991, Moscow, Russia.
Moscow Institute of Physics and Technology, Institutskiy per., 9, Dolgoprudny, 141700, Moscow Region, Russia.

Elnara Saffiulina (E)

A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilova Str., 28, 119991, Moscow, Russia.
Mendeleev University of Chemical Technology of Russia, Miusskaya pl., 9, 125047, Moscow, Russia.

Rinat Aysin (R)

A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilova Str., 28, 119991, Moscow, Russia.
Moscow Institute of Physics and Technology, Institutskiy per., 9, Dolgoprudny, 141700, Moscow Region, Russia.

Pavel Dorovatovskii (P)

National Research Centre "Kurchatov Institute", Akademika Kurchatova pl., 1, 123182, Moscow, Russia.

Lydia Nodaraki (L)

University of Manchester, Oxford Rd., Manchester, M13 9PL, UK.

Floriana Tuna (F)

University of Manchester, Oxford Rd., Manchester, M13 9PL, UK.

Yulia Nelyubina (Y)

A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilova Str., 28, 119991, Moscow, Russia.
Bauman Moscow State Technical University, 2nd Baumanskaya Str. 5, 105005, Moscow, Russia.

Classifications MeSH