A Nontoxic Bifunctional (Anti)Solvent as Digestive-Ripening Agent for High-Performance Perovskite Solar Cells.
antisolvents
digestive ripening
methyl benzoate
perovskites
solvents
thermal annealing
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Apr 2020
Apr 2020
Historique:
received:
30
10
2019
revised:
21
01
2020
pubmed:
23
2
2020
medline:
23
2
2020
entrez:
22
2
2020
Statut:
ppublish
Résumé
The preparation of high-quality perovskite films is important for achieving high-performance perovskite solar cells (PSCs). The effective balance between solvent and antisolvent is an essential factor for regulating high-quality perovskite film during the spin-coating and thermal-annealing steps. In this work, a greener, nonhalogenated, nontoxic bifunctional (anti)solvent, methyl benzoate (MB), is developed not only as an antisolvent to rapidly generate crystal seeds at the perovskite spin-coating step, but also as a digestive-ripening solvent for the perovskite precursors, which can prevent the loss of organic components during the thermal-annealing stage and effectively suppress the formation of miscellaneous lead halide phases. As a result, this novel bifunctional (anti)solvent is employed in planar n-i-p PSCs for engineering high-quality perovskite layers and thus achieving a power conversion efficiency up to 22.37% with negligible hysteresis and >1300 h stability. Moreover, due to the high boiling point and low-volatility characteristic of MB, high-performance PSCs are achieved reproducibly at different operating temperatures (22-34 °C). Therefore, this developed bifunctional solvent system can provide a promising platform toward globally upscaling and commercializing PSCs in all seasons and regions.
Identifiants
pubmed: 32083790
doi: 10.1002/adma.201907123
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e1907123Subventions
Organisme : National Key Research and Development Program of China
ID : 2017YFE0131900
Organisme : National Key Research and Development Program of China
ID : 2017YFB0404500
Organisme : National Natural Science Foundation of China
ID : 91833306
Organisme : National Natural Science Foundation of China
ID : 91733302
Organisme : National Natural Science Foundation of China
ID : 21601085
Informations de copyright
© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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