Overcoming the Interfacial Limitations Imposed by the Solid-Solid Interface in Solid-State Batteries Using Ionic Liquid-Based Interlayers.
Li dendrites
Li garnet
bipolar cells
interfacial modifications
ionic liquids
solid-electrolytes
solid-state batteries
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
Apr 2020
Apr 2020
Historique:
received:
14
01
2020
pubmed:
28
2
2020
medline:
28
2
2020
entrez:
28
2
2020
Statut:
ppublish
Résumé
Li-garnets are promising inorganic ceramic solid electrolytes for lithium metal batteries, showing good electrochemical stability with Li anode. However, their brittle and stiff nature restricts their intimate contact with both the electrodes, hence presenting high interfacial resistance to the ionic mobility. To address this issue, a strategy employing ionic liquid electrolyte (ILE) thin interlayers at the electrodes/electrolyte interfaces is adopted, which helps overcome the barrier for ion transport. The chemically stable ILE improves the electrodes-solid electrolyte contact, significantly reducing the interfacial resistance at both the positive and negative electrodes interfaces. This results in the more homogeneous deposition of metallic lithium at the negative electrode, suppressing the dendrite growth across the solid electrolyte even at high current densities of 0.3 mA cm
Identifiants
pubmed: 32105407
doi: 10.1002/smll.202000279
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2000279Subventions
Organisme : Alexander-von-Humboldt Foundation
Organisme : Federal Ministry of Education and Research
ID : 03XP0175B
Organisme : Federal Ministry of Education and Research
ID : 03XP0138A-C
Organisme : Federal Ministry of Education and Research
ID : 03XP0225D
Informations de copyright
© 2020 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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