Interplay of Electronic and Steric Effects to Yield Low-Temperature CO Oxidation at Metal Single Sites in Defect-Engineered HKUST-1.
MOFs
density functional theory
dioxygen activation
reaction mechanism
single-atom sites
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
22 Jun 2020
22 Jun 2020
Historique:
received:
08
01
2020
revised:
18
03
2020
pubmed:
21
3
2020
medline:
21
3
2020
entrez:
21
3
2020
Statut:
ppublish
Résumé
In contrast to catalytically active metal single atoms deposited on oxide nanoparticles, the crystalline nature of metal-organic frameworks (MOFs) allows for a thorough characterization of reaction mechanisms. Using defect-free HKUST-1 MOF thin films, we demonstrate that Cu
Identifiants
pubmed: 32196128
doi: 10.1002/anie.202000385
pmc: PMC7318571
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
10514-10518Subventions
Organisme : Deutsche Forschungsgemeinschaft
ID : 3DMM2O
Informations de copyright
© 2020 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA.
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