Polymer Lamellae as Reaction Intermediates in the Formation of Copper Nanospheres as Evidenced by In Situ X-ray Studies.

coordination polymers copper formation mechanisms in situ X-ray measurements nanocrystals

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
06 Jul 2020
Historique:
received: 19 03 2020
pubmed: 22 4 2020
medline: 22 4 2020
entrez: 22 4 2020
Statut: ppublish

Résumé

The classical nucleation theory (CNT) is the most common theoretical framework used to explain particle formation. However, nucleation is a complex process with reaction pathways which are often not covered by the CNT. Herein, we study the formation mechanism of copper nanospheres using in situ X-ray absorption and scattering measurements. We reveal that their nucleation involves coordination polymer lamellae as pre-nucleation structures occupying a local minimum in the reaction energy landscape. Having learned this, we achieved a superior monodispersity for Cu nanospheres of different sizes. This report exemplifies the importance of developing a more realistic picture of the mechanism involved in the formation of inorganic nanoparticles to develop a rational approach to their synthesis.

Identifiants

pubmed: 32315499
doi: 10.1002/anie.202004081
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

11627-11633

Subventions

Organisme : Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung
ID : PYAPP2_166897/1
Organisme : H2020 Marie Skłodowska-Curie Actions
ID : 753124
Organisme : Bundesministerium für Bildung, Wissenschaft, Forschung und Technologie
ID : 05K19WM

Informations de copyright

© 2020 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

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Auteurs

Valeria Mantella (V)

Department of Chemical Sciences and Engineering, EPFL Valais Wallis, 1951, Sion, Switzerland.

Michal Strach (M)

Department of Chemical Sciences and Engineering, EPFL Valais Wallis, 1951, Sion, Switzerland.

Kilian Frank (K)

Department of Physics and Center for Nanoscience (CeNs), Ludwig-Maximilians Universität München, Germany.

James R Pankhurst (JR)

Department of Chemical Sciences and Engineering, EPFL Valais Wallis, 1951, Sion, Switzerland.

Dragos Stoian (D)

Department of Chemical Sciences and Engineering, EPFL Valais Wallis, 1951, Sion, Switzerland.

Chethana Gadiyar (C)

Department of Chemical Sciences and Engineering, EPFL Valais Wallis, 1951, Sion, Switzerland.

Bert Nickel (B)

Department of Physics and Center for Nanoscience (CeNs), Ludwig-Maximilians Universität München, Germany.

Raffaella Buonsanti (R)

Department of Chemical Sciences and Engineering, EPFL Valais Wallis, 1951, Sion, Switzerland.

Classifications MeSH