High-Rate Printing of Micro/Nanoscale Patterns Using Interfacial Convective Assembly.
Marangoni flow
convection
directed assembly
nanoparticles
printing
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Jun 2020
Jun 2020
Historique:
received:
02
02
2020
revised:
17
03
2020
accepted:
18
03
2020
pubmed:
24
4
2020
medline:
24
4
2020
entrez:
24
4
2020
Statut:
ppublish
Résumé
Printing of electronics has been receiving increasing attention from academia and industry over the recent years. However, commonly used printing techniques have limited resolution of micro- or sub-microscale. Here, a directed-assembly-based printing technique, interfacial convective assembly, is reported, which utilizes a substrate-heating-induced solutal Marangoni convective flow to drive particles toward patterned substrates and then uses van der Waals interactions as well as geometrical confinement to trap the particles in the pattern areas. The influence of various assembly parameters including type of mixing solvent, substrate temperature, particle concentration, and assembly time is investigated. The results show successful assembly of various nanoparticles in patterns of different shapes with a high resolution down to 25 nm. In addition, the assembly only takes a few minutes, which is two orders of magnitude faster than conventional convective assembly. Small-sized (diameter below 5 nm) nanoparticles tend to coalesce during the assembly process and form sintered structures. The fabricated silver nanorods show single-crystal structure with a low resistivity of 8.58 × 10
Identifiants
pubmed: 32323404
doi: 10.1002/adma.202000747
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2000747Subventions
Organisme : National Science Foundation Nanoscale Science and Engineering Center
ID : EEC-0832785
Organisme : Massachusetts Technology Collaborative
Informations de copyright
© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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