Light Tailoring of Internal Atomic Structure of Gold Nanorods.
atomic structure control
gold nanorods
light tailoring
ultrafast lasers
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
Jun 2020
Jun 2020
Historique:
received:
21
02
2020
revised:
29
03
2020
pubmed:
25
4
2020
medline:
25
4
2020
entrez:
25
4
2020
Statut:
ppublish
Résumé
Laser processing of gold nanorods (Au NRs) relying on light-matter interaction provides great opportunities in various potential applications. Unveiling the light-induced structure change is a crucial goal in order to control the shape and related properties for practical application. However, the internal atomic structure control of metallic NRs has long been a challenge. Here, the concept of internal atomic structure tailored with light is demonstrated and Au NRs with various internal atomic structures including point defects, twin structures, and polycrystalline nanospheres are fabricated. Experimental characterization and theoretical simulation show that light-induced localized energy deposition and dynamic stresses distribution give rise to atomic structure change. Au NRs with internal defects show enhanced potential to improve activity. The concept of light tailoring of internal atomic structure represents a promising strategy for the rational design of metallic NRs to boost wide applications.
Identifiants
pubmed: 32329236
doi: 10.1002/smll.202001101
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2001101Subventions
Organisme : National Key Research and Development Program of China
ID : 2017YFB1104300
Organisme : National Key Research and Development Program of China
ID : 2018YFB1107200
Organisme : National Natural Science Foundation of China
ID : 51775303
Organisme : Beijing Institute of Technology
Informations de copyright
© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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