A Superlattice-Stabilized Layered Oxide Cathode for Sodium-Ion Batteries.
layered cathodes
layered oxides
sodium-ion batteries
superlattices
transition-metal migration
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Jun 2020
Jun 2020
Historique:
received:
03
12
2019
revised:
15
03
2020
accepted:
30
03
2020
pubmed:
28
4
2020
medline:
28
4
2020
entrez:
28
4
2020
Statut:
ppublish
Résumé
Sodium-ion batteries are in high demand for large-scale energy storage applications. Although it is the most prevalent cathode, layered oxide is associated with significant undesirable characteristics, such as multiple plateaus in the charge-discharge profiles, and cation migration during repeated cycling of Na-ions insertion and extraction, which results in sluggish kinetics, capacity loss, and structural deterioration. Here, a new strategy, i.e., the manipulation of transition-metal ordering in layered oxides, is proposed to show a prolonged charge-discharge plateau and cation-migration-free structural evolution. The results demonstrate that the transition-metal ordering with a honeycomb-type superlattice can adjust the crystal lattice and suppress cation migration by modifying the crystal strain to realize a large reversible capacity and excellent cycling performance, which are not characteristics of the widely used common layered oxides. These findings can provide new insight that can be used to improve the design of high-performance electrode materials for secondary-ion batteries.
Identifiants
pubmed: 32338396
doi: 10.1002/adma.201907936
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e1907936Subventions
Organisme : National Key Research and Development Program of China
ID : 2016YFB0100203
Organisme : Natural Science Foundation of Jiangsu Province
ID : BK20170630
Organisme : National Natural Science Foundation of China
ID : 51602144
Organisme : National Natural Science Foundation of China
ID : 21403107
Organisme : National Natural Science Foundation of China
ID : 21673116
Organisme : National Natural Science Foundation of China
ID : 51902193
Informations de copyright
© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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