Electrocatalytically Active Fe-(O-C

ammonia electrocatalysis nitrogen reduction single-atom catalysts

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
03 Aug 2020
Historique:
received: 23 04 2020
pubmed: 6 5 2020
medline: 6 5 2020
entrez: 6 5 2020
Statut: ppublish

Résumé

Single-atom catalysts have demonstrated their superiority over other types of catalysts for various reactions. However, the reported nitrogen reduction reaction single-atom electrocatalysts for the nitrogen reduction reaction exclusively utilize metal-nitrogen or metal-carbon coordination configurations as catalytic active sites. Here, we report a Fe single-atom electrocatalyst supported on low-cost, nitrogen-free lignocellulose-derived carbon. The extended X-ray absorption fine structure spectra confirm that Fe atoms are anchored to the support via the Fe-(O-C

Identifiants

pubmed: 32367577
doi: 10.1002/anie.202005930
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

13423-13429

Subventions

Organisme : National Natural Science Foundation of China
ID : 51432009
Organisme : National Natural Science Foundation of China
ID : 51872292
Organisme : National Natural Science Foundation of China
ID : 11874334
Organisme : Youth Innovation Promotion Association of Chinese Academy of Sciences
ID : 2020458

Informations de copyright

© 2020 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

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Auteurs

Shengbo Zhang (S)

Key Laboratory of Materials Physics, Centre for Environmental and Energy Nanomaterials, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, Anhui, 230031, China.
University of Science and Technology of China, Hefei, Anhui, 230031, China.

Meng Jin (M)

Key Laboratory of Materials Physics, Centre for Environmental and Energy Nanomaterials, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, Anhui, 230031, China.
University of Science and Technology of China, Hefei, Anhui, 230031, China.

Tongfei Shi (T)

Key Laboratory of Materials Physics, Centre for Environmental and Energy Nanomaterials, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, Anhui, 230031, China.

Miaomiao Han (M)

Key Laboratory of Materials Physics, Centre for Environmental and Energy Nanomaterials, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, Anhui, 230031, China.

Qiao Sun (Q)

State Key Laboratory of Radiation Medicine and Protection, Collaborative Innovation Centre of Radiation Medicine of Jiangsu Higher Education Institutes, School for Radiological and Interdisciplinary Sciences, Soochow University, Suzhou, 215123, China.

Yue Lin (Y)

Hefei National Laboratory for Physical Sciences at the Microscale University of Science and Technology of China, Hefei, 230026, China.

Zhenhua Ding (Z)

Anhui Insitute of Product Quality Supervision and Inspection, Hefei, 230026, China.

Li Rong Zheng (LR)

Beijing Synchrotron Radiation Facility, Institute of High Energy Physics, Chinese Academy of Sciences, 19B Yuquan Road, Beijing, 100049, China.

Guozhong Wang (G)

Key Laboratory of Materials Physics, Centre for Environmental and Energy Nanomaterials, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, Anhui, 230031, China.

Yunxia Zhang (Y)

Key Laboratory of Materials Physics, Centre for Environmental and Energy Nanomaterials, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, Anhui, 230031, China.

Haimin Zhang (H)

Key Laboratory of Materials Physics, Centre for Environmental and Energy Nanomaterials, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, Anhui, 230031, China.

Huijun Zhao (H)

Key Laboratory of Materials Physics, Centre for Environmental and Energy Nanomaterials, Anhui Key Laboratory of Nanomaterials and Nanotechnology, CAS Center for Excellence in Nanoscience, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, Anhui, 230031, China.
Centre for Clean Environment and Energy Energy, Griffith University, Gold Coast Campus, QLD, 4222, Australia.

Classifications MeSH