Structural peculiarities of lysozyme - PLURONIC complexes at the aqueous-air and liquid-liquid interfaces and in the bulk of aqueous solution.

Lysozyme Lysozyme-Pluronic complex Pluronic copolymers

Journal

International journal of biological macromolecules
ISSN: 1879-0003
Titre abrégé: Int J Biol Macromol
Pays: Netherlands
ID NLM: 7909578

Informations de publication

Date de publication:
05 May 2020
Historique:
received: 25 02 2020
revised: 23 04 2020
accepted: 24 04 2020
pubmed: 11 5 2020
medline: 11 5 2020
entrez: 11 5 2020
Statut: aheadofprint

Résumé

Interaction between proteins and synthetic polymers that represent a perspective potential in drug delivery or/and already used in medicine plays a key role in biological functioning of both molecules along with a system as a whole. In present study association between hen egg white lysozyme and Pluronic triblock-copolymers (L121, P123 and F127) in the bulk of the solution as well as at the aqueous-air and liquid-liquid interfaces was analyzed by means of spectroscopic and radiochemical assay. In protein-Pluronic complexes lysozyme keeps the secondary structure (CD and SAXS data results), while fluorescence and UV-analysis indicates changes in the local surrounding of fluorophoric amino acid residues. Radiochemical assay in combination with molecular docking reveals the formation of the complexes, in which proline residues turned to the interface between water and hydrophobic medium.

Identifiants

pubmed: 32387357
pii: S0141-8130(20)33088-9
doi: 10.1016/j.ijbiomac.2020.04.221
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

721-731

Informations de copyright

Copyright © 2020 Elsevier B.V. All rights reserved.

Auteurs

Maria G Chernysheva (MG)

Dpt. Chemistry, Lomonosov Moscow State University, 119991 Moscow, Russia. Electronic address: chernysheva@radio.chem.msu.ru.

Alexey V Shnitko (AV)

Dpt. Chemistry, Lomonosov Moscow State University, 119991 Moscow, Russia.

Alexander L Ksenofontov (AL)

Belozersky Institute of Physico-Chemical Biology, Lomonosov Moscow State University, 119992, Moscow, Russia.

Alexander M Arutyunyan (AM)

Belozersky Institute of Physico-Chemical Biology, Lomonosov Moscow State University, 119992, Moscow, Russia.

Maxim V Petoukhov (MV)

A. V. Shubnikov Institute of Crystallography of Federal Scientific Research Centre "Crystallography and Photonics" of Russian Academy of Sciences, 119333 Moscow, Russia; A. N. Frumkin Institute of Physical Chemistry and Electrochemistry of Russian Academy of Sciences, 119071 Moscow, Russia.

Gennadii A Badun (GA)

Dpt. Chemistry, Lomonosov Moscow State University, 119991 Moscow, Russia.

Classifications MeSH