Nanoscale Correlations between Metal-Insulator Transition and Resistive Switching Effect in Metallic Perovskite Oxides.
complex oxides
memristor
metal-insulator transition
resistive switching
scanning probe microscopy
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
Jun 2020
Jun 2020
Historique:
received:
28
02
2020
revised:
30
03
2020
accepted:
31
03
2020
pubmed:
12
5
2020
medline:
12
5
2020
entrez:
12
5
2020
Statut:
ppublish
Résumé
Strongly correlated perovskite oxides are a class of materials with fascinating intrinsic physical functionalities due to the interplay of charge, spin, orbital ordering, and lattice degrees of freedom. Among the exotic phenomena arising from such an interplay, metal-insulator transitions (MITs) are fundamentally still not fully understood and are of large interest for novel nanoelectronics applications, such as resistive switching-based memories and neuromorphic computing devices. In particular, rare-earth nickelates and lanthanum strontium manganites are archetypical examples of bandwidth-controlled and band-filling-controlled MIT, respectively, which are used in this work as a playground to correlate the switching characteristics of the oxides and their MIT properties by means of local probe techniques in a systematic manner. These findings suggest that an electric-field-induced MIT can be triggered in these strongly correlated systems upon generation of oxygen vacancies and establish that lower operational voltages and larger resistance ratios are obtained in those films where the MIT lies closer to room temperature. This work demonstrates the potential of using MITs in the next generation of nanoelectronics devices.
Identifiants
pubmed: 32390240
doi: 10.1002/smll.202001307
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2001307Subventions
Organisme : Ministry of Economy and Competitiveness
Organisme : Programme for Centres of Excellence in R&D
ID : SEV-2015-0496
Organisme : CONSOLIDER Excellence Network
ID : MAT2015-68994-REDC
Organisme : CONSOLIDER Excellence Network
ID : MAT2014-56063-C2-1-R
Organisme : European Regional Development Fund
Organisme : Centro Superior de Investigaciones Científicas
Organisme : Catalan Government
ID : 2017-SGR-1519
Organisme : Spanish Ministry of Economy
ID : BES-2012-053814
Informations de copyright
© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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