Diagenetic production, accumulation and sediment-water exchanges of methylmercury in contrasted sediment facies of Lake Titicaca (Bolivia).

Diffusive fluxes Early diagenesis High altitude ecosystem Lake sediment Methylmercury

Journal

The Science of the total environment
ISSN: 1879-1026
Titre abrégé: Sci Total Environ
Pays: Netherlands
ID NLM: 0330500

Informations de publication

Date de publication:
25 Jun 2020
Historique:
received: 09 12 2019
revised: 18 03 2020
accepted: 19 03 2020
entrez: 13 5 2020
pubmed: 13 5 2020
medline: 13 5 2020
Statut: ppublish

Résumé

Monomethylmercury (MMHg) concentrations in aquatic biota from Lake Titicaca are elevated although the mercury (Hg) contamination level of the lake is low. The contribution of sediments to the lake MMHg pool remained however unclear. In this work, seven cores representative of the contrasted sediments and aquatic ecotopes of Lake Titicaca were sliced and analyzed for Hg and redox-sensitive elements (Mn, Fe, N and S) speciation in pore-water (PW) and sediment to document early diagenetic processes responsible for MMHg production and accumulation in PW during organic matter (OM) oxidation. The highest MMHg concentrations (up to 12.2 ng L

Identifiants

pubmed: 32392692
pii: S0048-9697(20)31601-6
doi: 10.1016/j.scitotenv.2020.138088
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

138088

Informations de copyright

Copyright © 2020 Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

S Guédron (S)

Univ. Grenoble Alpes, Univ. Savoie Mont Blanc, CNRS, IRD, IFSTTAR, ISTerre, 38000 Grenoble, France; Laboratorio de Hidroquímica, Instituto de Investigaciones Químicas, Universidad Mayor de San Andres, Campus Universitario de Cota Cota, casilla 3161, La Paz, Bolivia. Electronic address: stephane.guedron@ird.fr.

S Audry (S)

Géosciences Environnement Toulouse, UMR5563, IRD UR 154, Université Paul Sabatier, 14 Avenue Edouard Belin, 31400 Toulouse, France.

D Acha (D)

Unidad de Calidad Ambiental (UCA), Instituto de Ecología, Universidad Mayor de San Andrés, Campus Universitario de Cota Cota, casilla 3161, La Paz, Bolivia.

S Bouchet (S)

Universite de Pau et des Pays de l'Adour, E2S UPPA, CNRS, IPREM, Institut des Sciences Analytiques et de Physico-chimie pour l'Environnement et les matériaux, Pau, France.

D Point (D)

Géosciences Environnement Toulouse, UMR5563, IRD UR 154, Université Paul Sabatier, 14 Avenue Edouard Belin, 31400 Toulouse, France.

T Condom (T)

Univ. Grenoble Alpes, CNRS, IRD, Grenoble INP, Institut des Géosciences de l'Environnement (IGE), UMR 5001, F-38000 Grenoble, France.

C Heredia (C)

Univ. Grenoble Alpes, Univ. Savoie Mont Blanc, CNRS, IRD, IFSTTAR, ISTerre, 38000 Grenoble, France; Unidad de Calidad Ambiental (UCA), Instituto de Ecología, Universidad Mayor de San Andrés, Campus Universitario de Cota Cota, casilla 3161, La Paz, Bolivia.

S Campillo (S)

Univ. Grenoble Alpes, Univ. Savoie Mont Blanc, CNRS, IRD, IFSTTAR, ISTerre, 38000 Grenoble, France.

P A Baya (PA)

Géosciences Environnement Toulouse, UMR5563, IRD UR 154, Université Paul Sabatier, 14 Avenue Edouard Belin, 31400 Toulouse, France.

A Groleau (A)

Institut de Physique du Globe de Paris (IPGP), 1, rue Jussieu, 75238 Paris Cedex 05, France.

E Amice (E)

LEMAR- Laboratoire des sciences de l'environnement marin, Institut Universitaire Européen de la Mer - Technopôle Brest-Iroise, Rue Dumont d'Urville, 29280 Plouzané, France.

D Amouroux (D)

Unidad de Calidad Ambiental (UCA), Instituto de Ecología, Universidad Mayor de San Andrés, Campus Universitario de Cota Cota, casilla 3161, La Paz, Bolivia; Universite de Pau et des Pays de l'Adour, E2S UPPA, CNRS, IPREM, Institut des Sciences Analytiques et de Physico-chimie pour l'Environnement et les matériaux, Pau, France.

Classifications MeSH