VOCs adsorption on activated carbon with initial water vapor contents: Adsorption mechanism and modified characteristic curves.

Carbon Characteristic adsorption curves Initial water vapor LSER Volatile organic compounds

Journal

The Science of the total environment
ISSN: 1879-1026
Titre abrégé: Sci Total Environ
Pays: Netherlands
ID NLM: 0330500

Informations de publication

Date de publication:
20 Aug 2020
Historique:
received: 13 03 2020
revised: 26 04 2020
accepted: 01 05 2020
pubmed: 14 5 2020
medline: 14 5 2020
entrez: 14 5 2020
Statut: ppublish

Résumé

In practice, regeneration of adsorbent is always achieved by heating with hot steam, leaving some water in the adsorbent bed, which may negatively affect the VOCs adsorption. In this research, adsorption isotherms of 12 VOCs (ketones, alkanes, alcohols, halohydrocarbons, and aromatic hydrocarbons) on granular activated carbon (GAC) with different initial water contents (IWC) were conducted. Adsorption interactions between VOCs and GAC at different IWC were investigated using the combination of Linear Solvation Energy Relationship (LSER) and Dubinin-Radushkevich (DR) equation. The results showed that initial water vapor could reduce adsorption capacities and partition coefficient of 12 VOCs, especially at low VOCs concentration. According to LSER, electron acceptor ability (∑β

Identifiants

pubmed: 32402907
pii: S0048-9697(20)32701-7
doi: 10.1016/j.scitotenv.2020.139184
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

139184

Informations de copyright

Copyright © 2020 Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Lijuan Jia (L)

State Key Laboratory of Pollution Control and Resource Reuse, School of the Environment, Nanjing University, 163 Xianlin Avenue, Nanjing 210023, China; Department of Applied Chemistry, Yuncheng University, 1155 Fudan West Street, Yuncheng 044000, China; Stockbridge School of Agriculture, University of Massachusetts, Amherst, MA 01003, USA.

Jialu Shi (J)

Key Laboratory for Yellow River and Huai River Water Environment and Pollution Control, Ministry of Education, Henan Key Laboratory for Environmental Pollution Control, School of Environment, Henan Normal University, Xinxiang 453007, China.

Chao Long (C)

State Key Laboratory of Pollution Control and Resource Reuse, School of the Environment, Nanjing University, 163 Xianlin Avenue, Nanjing 210023, China. Electronic address: clong@nju.edu.cn.

Fei Lian (F)

Institute of Environmental Processes and Pollution Control, School of Environmental and Civil Engineering, Jiangnan University, Wuxi 214122, China.

Baoshan Xing (B)

Stockbridge School of Agriculture, University of Massachusetts, Amherst, MA 01003, USA.

Classifications MeSH