Controlling factors for the distribution of typical organic pollutants in the surface sediment of a macrotidal bay.


Journal

Environmental science and pollution research international
ISSN: 1614-7499
Titre abrégé: Environ Sci Pollut Res Int
Pays: Germany
ID NLM: 9441769

Informations de publication

Date de publication:
Aug 2020
Historique:
received: 26 11 2019
accepted: 05 05 2020
pubmed: 18 5 2020
medline: 11 7 2020
entrez: 17 5 2020
Statut: ppublish

Résumé

Marine sediment is the final sink of polycyclic aromatic hydrocarbons (PAHs) from river input and atmospheric deposition. Such kind of pollutant cycles in the marine environment is usually controlled by hydrodynamic conditions. Many previous studies have explored how ocean currents influence pollutant distribution, but very few studies have focused on the relationships between the distribution patterns of pollutant and residual currents or sediment transport. In this study, 16 monomers of PAHs from 135 surface sediment samples collected in the Hangzhou Bay, a typical macrotidal bay, were systematically identified and their sources were analyzed. The sediment characteristics and distribution pattern were also comprehensively analyzed. The results showed the seabed sediments were moderately polluted by PAHs with a level of 38.58-1371.06 ng/g (median 186.70 ng/g). Most of the PAHs are composed of three to five rings, originated from combustion of coal and firewood. The combustion of oil also contributes to PAHs in seabed sediments for some areas. The PAHs are found to be concentrated within the estuary and the offshore areas, as well in coastal ocean. Fine-grained sediment transport is controlled by residual currents, which leads to PAH accumulation in the bay and the offshore areas, forming a high-value distribution pattern. Hence, we conclude that residual current is the main factors that control the long-term distribution of PAHs in the seabed sediments of the macrotidal bay. Temporal and spatial varying models of PAHs were needed in a further study to explore further the mechanisms how PAHs are transported in coastal areas.

Identifiants

pubmed: 32415449
doi: 10.1007/s11356-020-09199-w
pii: 10.1007/s11356-020-09199-w
doi:

Substances chimiques

Environmental Pollutants 0
Polycyclic Aromatic Hydrocarbons 0
Water Pollutants, Chemical 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

28276-28287

Subventions

Organisme : National Natural Science Foundation of China
ID : 41625021

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Auteurs

Ning Wang (N)

Ministry of Education Key Laboratory for Coast and Island Development, School of Geographic and Oceanographic Sciences, Nanjing University, Nanjing, 210093, China.

Ya Ping Wang (YP)

Ministry of Education Key Laboratory for Coast and Island Development, School of Geographic and Oceanographic Sciences, Nanjing University, Nanjing, 210093, China. ypwang@nju.edu.cn.
State Key Laboratory of Estuarine and Coastal Research, School of Marine Sciences, East China Normal University, Shanghai, 200241, China. ypwang@nju.edu.cn.

Xiaoyong Duan (X)

Qingdao Institute of Marine Geology, China Geological Survey, Qingdao, 266071, China. duan-x@foxmail.com.

Jianqiang Wang (J)

Zhejiang Institute of Hydrogeology and Engineering Geology, Zhejiang, 315012, China.

Yongqing Xie (Y)

Zhejiang Institute of Hydrogeology and Engineering Geology, Zhejiang, 315012, China.

Chao Dong (C)

Zhejiang Institute of Hydrogeology and Engineering Geology, Zhejiang, 315012, China.

Jianhua Gao (J)

Ministry of Education Key Laboratory for Coast and Island Development, School of Geographic and Oceanographic Sciences, Nanjing University, Nanjing, 210093, China.

Ping Yin (P)

Qingdao Institute of Marine Geology, China Geological Survey, Qingdao, 266071, China.

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